We introduce a thermodynamical model based on the two-temperature approach in order to fully understand the dynamics of the coherent A(1g) phonon in laser-excited bismuth. Using this model, we simulate the time evolution of (111) Bragg peak intensities measured by Fritz et al. [Science 315, 633 (2007)] in femtosecond x-ray diffraction experiments performed on a bismuth film for different laser fluences. The agreement between theoretical and experimental results is striking not only because we use fluences very close to the experimental ones but also because most of the model parameters are obtained from ab initio calculations performed for different electron temperatures.
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http://dx.doi.org/10.1103/PhysRevLett.106.155503 | DOI Listing |
We demonstrate a noninvasive time-sorting method for ultrafast electron diffraction (UED) experiments with radio frequency (rf)-compressed electron beams. We show that electron beam energy and arrival time at the sample after the rf compression are strongly correlated, such that the arrival time jitter may be corrected through the measurement of the beam energy. The method requires minimal change to the infrastructure of most of the UED machines and is applicable to both keV and MeV UED.
View Article and Find Full Text PDFPhys Rev Lett
April 2011
Institut de Physique de Rennes, UMR UR1-CNRS 6251, Campus de Beaulieu-Bat 11 A, 35042 Rennes Cedex, France, EU.
We introduce a thermodynamical model based on the two-temperature approach in order to fully understand the dynamics of the coherent A(1g) phonon in laser-excited bismuth. Using this model, we simulate the time evolution of (111) Bragg peak intensities measured by Fritz et al. [Science 315, 633 (2007)] in femtosecond x-ray diffraction experiments performed on a bismuth film for different laser fluences.
View Article and Find Full Text PDFOpt Express
September 2010
School of Mechanical Engineering, Purdue University, West Lafayette, IN 47907, USA.
For semimetals such as bismuth, ultrafast femtosecond laser-excited coherent phonons at laser fluences below the damage threshold have been studied extensively. In this work, we investigate whether or not coherent phonon oscillations contribute to material's permanent damage, or can enhance or suppress such damage. We employed temporally-shaped femtosecond pulses to either enhance or cancel coherent phonon oscillations.
View Article and Find Full Text PDFPhys Rev Lett
April 2008
Paul Scherrer Institut, CH-5232 Villigen PSI, Switzerland.
We employ grazing-incidence femtosecond x-ray diffraction to characterize the coherent, femtosecond laser-induced lattice motion of a bismuth crystal as a function of depth from the surface with a temporal resolution of 193+/-8 fs. The data show direct consequences on the lattice motion from carrier diffusion and electron-hole interaction, allowing us to estimate an effective diffusion rate of D=2.3+/-0.
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