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Hierarchical-Porous Hollow Nitrogen-Doped Carbon-Supported Pt Alloy Catalysts with a Controllable Triheterointerface for Methanol Electrooxidation.
ACS Appl Mater Interfaces
January 2025
School of Chemistry and Chemical Engineering, Beijing Institute of Technology, Beijing 100081, China.
Carbon-supported Pt-based catalysts are the most effective catalysts for direct methanol fuel cells (DMFCs). However, challenges such as high Pt loading, cost, and susceptibility to CO poisoning severely hinder the development of DMFCs. In this paper, CoFeO@polymer@ZIF-67 is prepared successfully through sequential solution polymerization and in situ growth with modified CoFeO as the core.
View Article and Find Full Text PDFThe synergistic interaction effect between biochar and plant growth-promoting rhizobacteria on beneficial microbial communities in soil.
Front Plant Sci
December 2024
College of Plant Protection, Yunnan Agricultural University, Kunming, China.
Excessive use of chemical fertilizers and extensive farming can degrade soil properties so that leading to decline in crop yields. Combining plant growth-promoting rhizobacteria (PGPR) with biochar (BC) may be an alternative way to mitigate this situation. However, the proportion of PGPR and BC at which crop yield can be improved, as well as the improvement effect extent on different eco-geographic region and crops, remain unclear.
View Article and Find Full Text PDFRadiocarbon monoxide indicates increasing atmospheric oxidizing capacity.
Nat Commun
January 2025
National Institute of Water and Atmospheric Research (NIWA), 301 Evans Bay Parade, Wellington, 6021, New Zealand.
Hydroxyl (OH) is the atmosphere's main oxidant removing most pollutants including methane. Its short lifetime prevents large-scale direct observational quantification. Abundances inferred using anthropogenic trace gas measurements and models yield conflicting trend estimates.
View Article and Find Full Text PDFUnderstanding the Scope of Cytochrome P450-Catalyzed Radical Dimerization of Diketopiperazines.
Biochemistry
January 2025
Department of Pharmaceutical Sciences, University of Shizuoka, Shizuoka 422-8526, Japan.
DtpC was isolated from the ditryptophenaline biosynthetic pathway found in filamentous fungi as a cytochrome P450 (P450) that catalyzes the dimerization of diketopiperazines. More recently, several similar P450s were discovered. While a vast majority of such P450s generate asymmetric diketopiperazine dimers, DtpC and other fungal P450s predominantly catalyze the formation of symmetric dimer products.
View Article and Find Full Text PDFGeneral synthesis of neighboring dual-atomic sites with a specific pre-designed distance via an interfacial-fixing strategy.
Nat Commun
January 2025
Anhui University of Technology, Ma'anshan, Anhui, 243002, P. R. China.
A potential non-precious metal catalyst for oxygen reduction reaction should contain metal-N moieties. However, most of the current strategies to regulate the distances between neighboring metal sites are not pre-designed but depend on the probability by tuning the metal loading or the support. Herein, we report a general method for the synthesis of neighboring metal-N moieties (metal = Fe, Cu, Co, Ni, Zn, and Mn) via an interfacial-fixing strategy.
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