Effect of Bi doping on magnetoresistance in La(0.7-x) Bi(x)Sr0.3MnO3.

J Nanosci Nanotechnol

Department of Physics and NUS Nanoscience and Nanotechnology Initiative (NUSNNI), 2 Science Drive 3, Faculty of Science, National University of Singapore-117542, Singapore.

Published: March 2011

It is shown that upon increasing Bi content (x) in La(0.7-x)Bi(x)Sr0.3MnO3, the ground state changes from ferromagnetic metal (x = 0) to charge ordered antiferromagnetic insulator (x > 0.4). The x = 0.3 compound shows unusual magnetic and magnetoresistive properties: it shows hysteresis in magnetization as a function of temperature, field-induced metamagnetic transition in the paramagnetic state, and nearly 100% magnetoresistance. The magnetoresistance as a function of composition at microH = 5 T increases from 38% for x = 0.05 to 99.6% for x = 0.3 and then drops to 60% for x = 0.4. The unusual behavior of x = 0.3 composition is suggested to coexistence of short-range charge-ordered clusters and ferromagnetic domains. The field-induced melting of these charge-ordered clusters leads to large magnetoresistance effect.

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http://dx.doi.org/10.1166/jnn.2011.2701DOI Listing

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