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Highly 002-Oriented Dendrite-Free Anode Achieved by Enhanced Interfacial Electrostatic Adsorption for Aqueous Zinc-Ion Batteries.
ACS Nano
August 2024
State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Dalian 116023 (China).
Rechargeable aqueous zinc-ion batteries (AZIBs) are gaining recognition as promising next-generation energy storage solution, due to their intrinsic safety and low cost. Nevertheless, the advancement of AZIBs is greatly limited by the abnormal growth of zinc dendrites during cycling. Electrolyte additives are effective at suppressing zinc dendrites, but there is currently no effective additive screening criterion.
View Article and Find Full Text PDFAn integrated self-optimizing programmable chemical synthesis and reaction engine.
Nat Commun
February 2024
School of Chemistry, The University of Glasgow, University Avenue, Glasgow, G12 8QQ, UK.
Article Synopsis
- Rapid advancements in robotic platforms for chemistry are hindered by their current inability to adapt to changing conditions in real-time.
- A new dynamically programmable system has been developed that uses seven sensors to monitor reactions continuously, enabling it to optimize and discover new molecules efficiently.
- The system successfully demonstrated closed-loop optimization through in-line spectroscopy techniques, resulting in significant yield improvements and the discovery of new reactions and molecules.
Self-Optimizing Flow Reactors Get a Boost by Multitasking.
ACS Cent Sci
May 2023
Center for Continuous Flow Synthesis and Processing (CC FLOW), Research Center Pharmaceutical Engineering GmbH (RCPE), Inffeldgasse 13, Graz 8010, Austria.
Environmentally adaptive MOF-based device enables continuous self-optimizing atmospheric water harvesting.
Nat Commun
August 2022
Materials Discovery Research Unit, Advanced Research Centre, Royal Scientific Society, Amman, 11941, Jordan.
Harvesting water vapor from desert, arid environments by metal-organic framework (MOF) based devices to deliver clean liquid water is critically dependent on environment and climate conditions. However, reported devices have yet been developed to adapt in real-time to such conditions during their operation, which severely limits water production efficiency and unnecessarily increases power consumption. Herein, we report and detail a mode of water harvesting operation, termed 'adaptive water harvesting', from which a MOF-based device is proven capable of adapting the adsorption and desorption phases of its water harvesting cycle to weather fluctuations throughout a given day, week, and month such that its water production efficiency is continuously optimized.
View Article and Find Full Text PDFSelf-optimizing parallel millifluidic reactor for scaling nanoparticle synthesis.
Chem Commun (Camb)
April 2020
Mork Family Department of Chemical Engineering and Materials Science, University of Southern California, 925 Bloom Walk, Los Angeles, California 90089-1211, USA.
We developed a 16-channel millifluidic reactor that uses a multiphase gas-liquid flow to continuously produce colloidal CsPbBr quantum dots with a throughtput of ∼1 L h. The optical properties of the product were monitored, and the reaction conditions were optimized in real time based on the in situ photoluminescence characteristics of the quantum dots.
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