We demonstrate chirped-pulse operation of a Cr : YAG passively mode-locked laser. Different operation regimes of the laser are extensively investigated in the vicinity of zero dispersion both experimentally and numerically. It is shown that for a given laser configuration, transition to the positive dispersion regime allows a 5-fold increase in the output pulse energy, which is otherwise limited by the onset of the multipulsing or 'chaotic' mode-locking. The output pulses have 1.4 ps duration and are compressible down to 120 fs in a 3 m piece of silica fiber, enabling supercontinuum generation in a nonlinear fiber. The spectrum shape and operation stability of the chirped-pulse regime depend strongly on the amount and shape of the intracavity dispersion. The numerical model predicts the existence of the minimum amount of the positive dispersion, above which the chirped-pulse regime can be realized. Once located, the chirped-pulse regime can be reliably reproduced and is sufficiently stable for applications.
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http://dx.doi.org/10.1088/1367-2630/10/8/083022 | DOI Listing |
We report on a high-energy, few-ps, continuous-wave pumped Ho:YLF regenerative amplifier (RA) operating in a chirped-pulse amplification arrangement. A three-stage optical parametric amplifier serves as versatile seed source emitting broadband pulses centered at 2050 nm. It provides seed pulses with 4 µJ energy within the Ho:YLF amplification bandwidth centered at 2051 nm.
View Article and Find Full Text PDFJ Chem Phys
September 2024
Department of Chemistry, University of Missouri, Columbia, Missouri 65203, USA.
This second paper in a series of two describes the chirped-pulse ice apparatus that permits the detection of buffer gas cooled molecules desorbed from an energetically processed ice using broadband mm-wave rotational spectroscopy. Here, we detail the lower ice stage developed to generate ices at 4 K, which can then undergo energetic processing via UV/VUV photons or high-energy electrons and which ultimately enter the gas phase via temperature-programmed desorption (TPD). Over the course of TPD, the lower ice stage is interfaced with a buffer gas cooling cell that allows for sensitive detection via chirped-pulse rotational spectroscopy in the 60-90 GHz regime.
View Article and Find Full Text PDFNat Commun
May 2024
University of Texas at Austin, 2515 Speedway C1600, Austin, TX, 78712, USA.
Laser-driven plasma accelerators provide tabletop sources of relativistic electron bunches and femtosecond x-ray pulses, but usually require petawatt-class solid-state-laser pulses of wavelength λ ~ 1 μm. Longer-λ lasers can potentially accelerate higher-quality bunches, since they require less power to drive larger wakes in less dense plasma. Here, we report on a self-injecting plasma accelerator driven by a long-wave-infrared laser: a chirped-pulse-amplified CO laser (λ ≈ 10 μm).
View Article and Find Full Text PDFWe present a compact nonlinear compression scheme for the generation of millijoule few-cycle pulses beyond 4 µm wavelength. For this purpose 95 fs pulses at 5 µm from a 1 kHz midwave-IR optical parametric chirped pulse amplifier (OPCPA) are spectrally broadened due to a self-phase modulation in ZnSe. The subsequent compression in a bulk material yields 53 fs pulses with 1.
View Article and Find Full Text PDFWe demonstrate a 417 W, 175 kHz Innoslab chirped pulse amplification laser compressible to short and clean 406 fs pulse duration. A spectral bandwidth (full width at half maximum, FWHM) of ∼3 nm was maintained at full pump power, and the pulses exhibited good pulse quality in a wide tunable pulse energy range from 1.7 mJ to a maximum of 2.
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