We report on the generation of approximately 30-fs ultraviolet pulses with approximately 10 microJ energy by means of four-wave optical parametric chirped pulse amplification in fused silica. The four-wave optical parametric amplifier is pumped by the second-harmonic of the Ti:sapphire laser and is seeded by visible broadband chirped signal pulses. The idler pulses are produced in the ultraviolet by four-wave mixing and are compressed in a medium with normal group velocity dispersion.
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http://dx.doi.org/10.1364/OE.18.016096 | DOI Listing |
ACS Photonics
January 2025
Cardiff University School of Physics and Astronomy, The Parade, Cardiff CF24 3AA, United Kingdom.
The field of chiral nanoparticles is rapidly expanding, yet measuring the chirality of single nano-objects remains a challenging endeavor. Here, we report a technique to detect chiro-optical effects in single plasmonic nanoparticles by means of phase-sensitive polarization-resolved four-wave mixing interferometric microscopy. Beyond conventional circular dichroism, the method is sensitive to the particle polarizability, in amplitude and phase.
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January 2025
Department of Electronics and Nanoengineering, Aalto University, Espoo, Finland.
Coherent broadband light generation has attracted massive attention due to its numerous applications ranging from metrology, sensing, and imaging to communication. In general, spectral broadening is realized via third-order and higher-order nonlinear optical processes (e.g.
View Article and Find Full Text PDFNanophotonics
August 2024
Facultad de Ciencias Exactas y Naturales, Departamento de Física, Universidad de Buenos Aires, 1428 Buenos Aires, Argentina.
Nanophotonics
August 2024
School of Microelectronics, Southern University of Science and Technology, Shenzhen, China.
Gallium phosphide (GaP) has been increasingly prioritized, fueled by the enormous demands in visible light applications such as biomedical and quantum technologies. GaP has garnered tremendous attention in nanophotonics thanks to its high refractive index, indirect bandgap width of 2.26 eV, lattice perfectly matched with silicon, and omnipotent and competitive nonlinear optical properties.
View Article and Find Full Text PDFPhys Rev Lett
November 2024
National Research Council of Canada, 100 Sussex Drive, Ottawa, Ontario K1N 5A2, Canada.
Strongly driven nonlinear optical processes such as spontaneous parametric down-conversion and spontaneous four-wave mixing can produce multiphoton nonclassical beams of light which have applications in quantum information processing and sensing. In contrast to the low-gain regime, new physical effects arise in a high-gain regime due to the interactions between the nonclassical light and the strong pump driving the nonlinear process. Here, we describe and experimentally observe a gain-induced group delay between the multiphoton pulses generated in a high-gain type-II spontaneous parametric down-conversion source.
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