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Steering the Absorption Configuration of Intermediates over Pd-Based Electrocatalysts toward Efficient and Stable CO Reduction.
J Am Chem Soc
January 2025
Department of Industrial and Systems Engineering, The Hong Kong Polytechnic University, Kowloon 999077, Hong Kong, China.
Palladium (Pd) catalysts are promising for electrochemical reduction of CO to CO but often can be deactivated by poisoning owing to the strong affinity of *CO on Pd sites. Theoretical investigations reveal that different configurations of *CO endow specific adsorption energies, thereby dictating the final performances. Here, a regulatory strategy toward *CO absorption configurations is proposed to alleviate CO poisoning by simultaneously incorporating Cu and Zn atoms into ultrathin Pd nanosheets (NSs).
View Article and Find Full Text PDFObjectives: Examine the feasibility, acceptability, and preliminary effects of the Telephone Acceptance and Commitment Therapy Intervention for Caregivers (TACTICs) on dementia caregivers' anxiety, depression, caregiver burden, suffering, and anticipatory grief.
Method: A 2-arm pilot randomized trial with dementia caregivers ≥ 21 years old with clinically elevated anxiety or anxiety-related functional interference. Two cohorts were recruited at the beginning and end of the first year of the COVID-19 pandemic.
Amorphization Stabilizes Te-Based Aqueous Batteries via Confining Free Water.
Angew Chem Int Ed Engl
January 2025
Laboratory of Advanced Materials, Aqueous Battery Center, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, School of Chemistry and Materials, Fudan University, Shanghai, 200433, P. R. China.
Tellurium (Te), with its rich valence states (-2 to +6), could endow aqueous batteries with potentially high specific capacity. However, achieving complete and stable hypervalent Te/Te electrochemistry in an aqueous environment poses significant challenges, owing to the sluggish reduction kinetics, easy dissolution of Te species, and a controversial energy storage mechanism. Herein, we demonstrate a crystallographic regulation strategy for robust aqueous Te redox electrochemistry.
View Article and Find Full Text PDFHealth impact assessment of urban and transport developments in Barcelona: A case study.
Health Place
January 2025
Barcelona Institute for Global Health (ISGlobal), Doctor Aiguader 88, 08003, Barcelona, Spain; Universitat Pompeu Fabra (UPF), Department of Experimental and Health Sciences, Doctor Aiguader 88, 08003, Barcelona, Spain; CIBER Epidemiología y Salud Pública (CIBERESP), Melchor Fernández Almagro, 3-5, 28029, Madrid, Spain. Electronic address:
Background: Urban spaces need to be rethought to address growing health and environmental challenges. Urban density and transport systems contribute significantly to air pollution, negatively impacting public health. Barcelona has begun a transformation by introducing the Superblock model, an urban development with proven health benefits.
View Article and Find Full Text PDFNovel empress SARANI optimization algorithm for active power loss reduction and voltage stability enhancement.
Heliyon
November 2024
Prasad V.Potluri Siddhartha Institute of Technology, Kanuru, Vijayawada, Andhra Pradesh, 520007, India.
This paper proposes Pomarine jaeger Optimization (PJO) algorithm, Tiger hunting Optimization (THO) Algorithm, Desert Reynard and Vixen Inspired Optimization (DRVIO) Algorithm, Lonchodidae optimization (LO) algorithm, Caracal optimization (CO) algorithm, Barasingha optimization (BO) algorithm, Amur leopard optimization (AO) algorithm and Empress SARANI Optimization Algorithm to solve the active power loss reduction problem. Regular actions of Pomarine jaeger have been emulated to model the PJO procedure. In THO algorithm, how the Tiger moves to capture the prey is imitated and formulated.
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