We study the effect of pure dephasing on a two-level system in strong coupling in the nonlinear regime with the single mode of a cavity. The photoluminescence spectrum of the cavity has a robust tendency to display triplet structures, instead of the expected Jaynes-Cummings pairs of doublets at the incommensurate frequencies +/- (square root n +/- square root (n-1)) for integer n. We discuss recent experimental works that may already manifest signatures of single photon nonlinearities.
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http://dx.doi.org/10.1364/OE.18.007002 | DOI Listing |
J Chem Phys
November 2024
Faculty of Mathematics and Physics, Charles University, Ke Karlovu 5, 121 16 Prague 2, Czech Republic.
J Chem Phys
September 2024
Dipartimento di Scienze Chimiche e Farmaceutiche, Università di Trieste, Via L. Giorgieri 1, 34127 Trieste, Italy.
We present a multiscale method coupling the theory of open quantum systems with real-time ab initio treatment of electronic structure to study hot-carrier dynamics in photoexcited plasmonic systems. We combine the Markovian Stochastic Schrödinger equation with an ab initio GW coupled to the Bethe-Salpeter (BSE) equation description of the electronic degrees of freedom, interacting with a metallic nanoparticle modeled classically according to the polarizable continuum model. We apply this methodology to study the effect of relaxation (T1) and pure dephasing (T2) times on the hot-carrier dynamics in a system composed of a quantum portion described at GW/BSE level, i.
View Article and Find Full Text PDFEntropy (Basel)
August 2024
Grupo de Informação Quântica e Física Estatística, Centro de Ciências Exatas e das Tecnologias, Universidade Federal do Oeste da Bahia-Campus Reitor Edgard Santos, Rua Bertioga, 892, Morada Nobre I, Barreiras 47810-059, BA, Brazil.
Sci Rep
July 2024
Dipartimento di Fisica e Astronomia "Ettore Majorana", Università di Catania, Via Santa Sofia 64, 95123, Catania, Italy.
Quantum control techniques are one of the most efficient tools for attaining high-fidelity quantum operations and a convenient approach for quantum sensing and quantum noise spectroscopy. In this work, we investigate dynamical decoupling while processing an entangling two-qubit gate based on an Ising-xx interaction, each qubit affected by pure dephasing classical correlated 1/f-noises. To evaluate the gate error, we used the Magnus expansion introducing generalized filter functions that describe decoupling while processing and allow us to derive an approximate analytic expression as a hierarchy of nested integrals of noise cumulants.
View Article and Find Full Text PDFJ Nonlinear Sci
July 2024
Department of Mathematics, University of Surrey, Guildford, UK.
Several methods in nonadiabatic molecular dynamics are based on Madelung's hydrodynamic description of nuclear motion, while the electronic component is treated as a finite-dimensional quantum system. In this context, the quantum potential leads to severe computational challenges and one often seeks to neglect its contribution, thereby approximating nuclear motion as classical. The resulting model couples classical hydrodynamics for the nuclei to the quantum motion of the electronic component, leading to the structure of a complex fluid system.
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