Spin-spiral states in undoped manganites: role of finite Hund's rule coupling.

Phys Rev Lett

Institute Lorentz for Theoretical Physics, Leiden University, P.O. Box 9506, 2300 RA Leiden, The Netherlands.

Published: January 2010

The experimental observation of multiferroic behavior in perovskite manganites with a spiral spin structure requires a clarification of the origin of these magnetic states and their relation to ferroelectricity. We show that spin-spiral phases with a diagonal wave vector and also an E-type phase exist for intermediate value of Hund's rule and the Jahn-Teller coupling in the orbitally ordered and insulating state of the standard two-band model Hamiltonian for manganites. Our results support the spin-current mechanism for ferroelectricity and present an alternative view to earlier conclusions where frustrating superexchange couplings were crucial to obtaining spin-spiral states.

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http://dx.doi.org/10.1103/PhysRevLett.104.017201DOI Listing

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