The development of a robust light source that emits one photon at a time will allow new technologies such as secure communication through quantum cryptography. Devices based on fluorescent dye molecules, quantum dots and carbon nanotubes have been demonstrated, but none has combined a high single-photon flux with stable, room-temperature operation. Luminescent centres in diamond have recently emerged as a stable alternative, and, in the case of nitrogen-vacancy centres, offer spin quantum bits with optical readout. However, these luminescent centres in bulk diamond crystals have the disadvantage of low photon out-coupling. Here, we demonstrate a single-photon source composed of a nitrogen-vacancy centre in a diamond nanowire, which produces ten times greater flux than bulk diamond devices, while using ten times less power. This result enables a new class of devices for photonic and quantum information processing based on nanostructured diamond, and could have a broader impact in nanoelectromechanical systems, sensing and scanning probe microscopy.
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http://dx.doi.org/10.1038/nnano.2010.6 | DOI Listing |
Analyst
December 2024
Institut de Recherche Interdisciplinaire (IRI), CNRS USR 3078, Université Lille1, Parc de la Haute Borne, 50 avenue de Halley, BP 70478, 59658 Villeneuve d'Ascq, France.
Expression of concern for 'An impedimetric immunosensor based on diamond nanowires decorated with nickel nanoparticles' by Palaniappan Subramanian , , 2014, , 1726-1731, https://doi.org/10.1039/C3AN02045B.
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December 2024
Institut de Recherche Interdisciplinaire (IRI), CNRS USR 3078, Université Lille1, Parc de la Haute Borne, 50 avenue de Halley, BP 70478, 59658 Villeneuve d'Ascq, France.
Expression of concern for 'Diamond nanowires modified with poly[3-(pyrrolyl)carboxylic acid] for the immobilization of histidine-tagged peptides' by Palaniappan Subramanian , , 2014, , 4343-4349, https://doi.org/10.1039/C4AN00146J.
View Article and Find Full Text PDFNat Commun
November 2024
Department of Materials Science and Engineering, City University of Hong Kong, Kowloon, Hong Kong SAR, 999077, China.
Manipulation C-C coupling pathway is of great importance for selective CO electroreduction but remain challenging. Herein, two model Cu-based catalysts, by modifying Cu nanowires with Ag nanoparticles (AgCu NW) and Ag single atoms (AgCu NW), respectively, are rationally designed for exploring the C-C coupling mechanisms in electrochemical CO reduction reaction (CORR). Compared to AgCu NW, the AgCu NW exhibits a more than 10-fold increase of C selectivity in CO reduction to ethanol, with ethanol-to-ethylene ratio increased from 0.
View Article and Find Full Text PDFNano Lett
November 2024
Department of Engineering Physics, Ecole Polytechnique de Montreal, C. P. 6079, Succ. Centre-Ville, Montréal, Québec H3C 3A7, Canada.
The work unravels the previously unexplored atomic-scale mechanism involving the interaction of phonons with crystal homointerfaces. Silicon nanowires with engineered isotopic content and crystal phases were chosen for this investigation. Crystal polytypism, manifested by the presence of both diamond cubic and rhombohedral phases within the same nanowire, provided a testbed to study the impact of phase homointerfaces on phonon transport.
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December 2024
Department of Chemistry, Hasselt University, Diepenbeek, 3590, Belgium.
Diamond nanomaterials are renowned for their exceptional properties, which include the inherent attributes of bulk diamond. Additionally, they exhibit unique characteristics at the nanoscale, including high specific surface areas, tunable surface structure, and excellent biocompatibility. These multifaceted attributes have piqued the interest of researchers globally, leading to an extensive exploration of various diamond nanostructures in a myriad of applications.
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