Due to their apparent complexity, diffuse fields are not commonly used by conventional structural health monitoring methodologies. However, recent theoretical and experimental studies have demonstrated that local Green's functions (GFs) can be estimated from the cross-correlation of elastic diffuse fields (CDFs) recorded between any points of a sensor grid and generated by sources located remotely from the monitoring area. Hence, this CDF technique effectively transforming each measurement point into a virtual elastic source, thus allowing to measure the local structural response (or GF). Theoretical and experimental studies are conducted to assess the broadband performance of the CDF technique for the extraction of low-frequency coherent Lamb waves (4-90 kHz) propagating in a thin aluminum plate of complex geometry using a scanning laser Doppler vibrometer. The coherent signal-to-noise ratio and the accuracy of the phase and group velocity measurements of the coherent A(0) mode obtained from CDF are also measured to quantify the influence of the spatio-temporal characteristics of the recorded diffuse field, the number and spatial configuration of the remote ultrasonic sources, and the influence of incoherent measurement noise (e.g., sensor noise). In addition, a criterion to assess the emergence rate of late coherent coda arrivals from CDF is also formulated.
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http://dx.doi.org/10.1121/1.3257602 | DOI Listing |
ACS Appl Mater Interfaces
January 2025
Institute for Theoretical Physics, Georg-August University of Göttingen, 37077 Göttingen, Germany.
A Single-Chain-in-Mean-Field (SCMF) algorithm was introduced to study block copolymer electrolytes in nonequilibrium conditions. This method self-consistently combines a particle-based description of the polymer with a generalized diffusion equation for the ionic fluxes, thus exploiting the time scale separation between fast ion motion and the slow polymer relaxation and self-assembly. We apply this computational method to study ion fluxes in electrochemical cells containing poly(ethylene oxide)-polystyrene (PEO-PS) block copolymers with added lithium salt.
View Article and Find Full Text PDFNat Commun
January 2025
Department of Biomedical Engineering, Duke University, Durham, NC, USA.
Acoustically probing biological tissues with light or sound, photoacoustic and ultrasound imaging can provide anatomical, functional, and/or molecular information at depths far beyond the optical diffusion limit. However, most photoacoustic and ultrasound imaging systems rely on linear-array transducers with elevational focusing and are limited to two-dimensional imaging with anisotropic resolutions. Here, we present three-dimensional diffractive acoustic tomography (3D-DAT), which uses an off-the-shelf linear-array transducer with single-slit acoustic diffraction.
View Article and Find Full Text PDFJ Colloid Interface Sci
January 2025
School of Materials Science and Engineering, Xiangtan University, Xiangtan 411105, China. Electronic address:
Lithium-sulfur batteries (LSBs) are considered as the most potential next-generation rechargeable energy storage devices due to their high theoretical energy density. However, the commercialization is severely hampered by the shuttle effect and sluggish sulfur redox kinetics of sulfur cathodes. Herein, we propose MoS/CN heterostructures as potential cathodes for LSBs.
View Article and Find Full Text PDFSoft Matter
January 2025
SUPA and School of Physics and Astronomy, The University of Edinburgh, Peter Guthrie Tait Road, Edinburgh EH9 3FD, UK.
Recent theory and experiments have shown how the buildup of a high-concentration polymer layer at a one-dimensional solvent-air interface can lead to an evaporation rate that scales with time as and that is insensitive to the ambient humidity. Using phase field modelling we show that this scaling law constitutes a naturally emerging robust regime, diffusion-limited evaporation (DLE). This regime dominates the dynamical state diagram of the system, which also contains regions of constant and arrested evaporation, confirming and extending understanding of recent experimental observations and theoretical predictions.
View Article and Find Full Text PDFResearch (Wash D C)
January 2025
Future Energy and Innovation Laboratory, Central European Institute of Technology, Brno University of Technology, Brno 61200, Czech Republic.
Microrobots enhance contact with pollutants through their movement and flow-induced mixing, substantially improving wastewater treatment efficiency beyond traditional diffusion-limited methods. g-CN is an affordable and environmentally friendly photocatalyst that has been extensively researched in various fields such as biomedicine and environmental remediation. However, compared to other photocatalytic materials like TiO and ZnO, which are widely used in the fabrication of micro- and nanorobots, research on g-CN for these applications is still in its early stages.
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