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Steady state and transient absorption spectroscopy in metal halide perovskites.
Chem Soc Rev
January 2025
School of Science, RMIT University, Melbourne, 3000, Australia.
Metal halide perovskites (MHPs) have emerged as the most promising materials due to superior optoelectronic properties and great applications spanning from photovoltaics to photonics. Absorption spectroscopy provides a broad and deep insight into the carrier dynamics of MHPs, and is a critical complement to fluorescence and scattering spectroscopy. However, absorption spectroscopy is often misunderstood or underestimated, being seen as UV-vis spectroscopy only, which can lead to various misinterpretations.
View Article and Find Full Text PDFOn-Chip Metamaterial-Enhanced Mid-Infrared Photodetectors with Built-In Encryption Features.
Adv Sci (Weinh)
January 2025
College of Physics and Optoelectronic Engineering, Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences, No. 1, Sub-Lane Xiangshan, Xihu District, Hangzhou, 310024, China.
The integration of mid-infrared (MIR) photodetectors with built-in encryption capabilities holds immense promise for advancing secure communications in decentralized networks and compact sensing systems. However, achieving high sensitivity, self-powered operation, and reliable performance at room temperature within a miniaturized form factor remains a formidable challenge, largely due to constraints in MIR light absorption and the intricacies of embedding encryption at the device level. Here, a novel on-chip metamaterial-enhanced, 2D tantalum nickel selenide (Ta₂NiSe₅)-based photodetector, meticulously designed with a custom-engineered plasmonic resonance microstructure to achieve self-powered photodetection in the nanoampere range is unveiled.
View Article and Find Full Text PDFUltra-compact quintuple-band terahertz metamaterial biosensor for enhanced blood cancer diagnostics.
PLoS One
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Faculty of Engineering (FOE), Multimedia University (MMU), Cyberjaya, Selangor, Malaysia.
Cancer and its diverse variations pose one of the most significant threats to human health and well-being. One of the most aggressive forms is blood cancer, originating from bone marrow cells and disrupting the production of normal blood cells. The incidence of blood cancer is steadily increasing, driven by both genetic and environmental factors.
View Article and Find Full Text PDFTerahertz Saturable Absorption across Charge Separation in Photoexcited Monolayer Graphene/MoS Heterostructure.
J Phys Chem Lett
January 2025
Key Laboratory of Materials Physics, Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences, Hefei 230031, China.
Unveiling the nonlinear interactions between terahertz (THz) electromagnetic waves and free carriers in two-dimensional materials is crucial for the development of high-field and high-frequency electronic devices. Herein, we investigate THz nonlinear transport dynamics in a monolayer graphene/MoS heterostructure using time-resolved THz spectroscopy with intense THz pulses as the probe. Following ultrafast photoexcitation, the interfacial charge transfer establishes a nonequilibrium carrier redistribution, leaving free holes in the graphene and trapping electrons in the MoS.
View Article and Find Full Text PDFRadar-Terahertz-Infrared Compatible Stealth Coaxial Silver Nanowire@Carbon Nano-Cable Aerogel.
Angew Chem Int Ed Engl
January 2025
Center for Bioinspired Science and Technology, Hangzhou International Innovation Institute, Beihang University, Hangzhou, 311115.
Achieving multi-spectrum compatible stealth in radar-terahertz-infrared bands with robust performance has great prospects for both military and civilian applications. However, the progress of materials encounters substantial challenges due to the significant variability in frequency coupling properties across different electromagnetic wave bands. Here, this work presents the design of a multi-scale structure and fabricates a lightweight aerogel (silver nanowire@carbon, AgNW@C) consisting of a regular coaxial nano-cable, with silver nanowire as the core and amorphous-graphitized hybrid carbon as the outer-layer.
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