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Nonlinear Refraction and Absorption in Polymers Used for Femtosecond Direct Laser Writing.

ACS Omega

January 2025

Instituto de Física de São Carlos, Universidade de São Paulo, São Carlos, SP 13560-970, Brasil.

Direct laser writing (DLW) has been recognized as a unique technique for three-dimensional (3D) prototyping with resolution beyond the diffraction limit. One trend in DLW technologies is the use of polymers, given their favorable mechanical properties and optical quality, rendering them promising for the next generation of nonlinear photonic devices. However, absorptive properties that facilitate DLW processes may also hinder the performance of polymers as all-optical devices.

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Tunable Multisoliton State Ultrafast Fiber Laser Based on NiSe and Generation of Vector Dual-Wavelength Solitons.

ACS Appl Mater Interfaces

January 2025

College of Optical, Mechanical and Electrical Engineering, Zhejiang A&F University, Lin'an 311300, China.

As a member of the chalcogenide family, NiSe exhibits a direct bandgap of 1.74 eV, making it a promising candidate for nonlinear optical devices. However, its potential in the near-infrared region of the telecommunication band has not been fully explored.

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We have proposed and demonstrated the generation of a high-repetition-rate ultrashort pulse with long-term stability and low noise based on a harmonic mode-locked (HML) figure-9 fiber laser. Different HML orders from the 2nd to the 13th are generated by adjusting the pump power, net dispersion, and wave plate angles. A 2-GHz HML pulse is obtained with a 155-MHz fundamental repetition rate in a Yb-doped fiber laser, and the corresponding supermode suppression level is as high as 50 dB.

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In this paper, a model of generating mid-infrared (MIR) ultrashort laser pulse through difference frequency generation (DFG) is established. The pulse evolution relationship among the pump, signal, and idler pulses during the DFG process, as well as the effects of crystal length, pulse energy of the pump and signal lights, pulse width, and other factors on the characteristics of the MIR pulse are explored. Furthermore, through simulations from the time domain to the frequency domain, the spectral characteristics and angular distribution of MIR were analyzed.

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A single-shot non-interferometric ultrashort-pulse measurement method based on the dispersion scan (d-scan) technique with a substantially extended time span for the pulses to be measured is presented. While single-shot d-scan is typically used for rather short femtosecond pulses, the presented multiple-reflections d-scan (MR d-scan) technique allows measurement of both short and long femtosecond pulses. Single-shot d-scan is currently limited to pulses with a maximum duration of 60 fs using a chromatic dispersion, i.

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