We report the first known demonstration of frequency-modulation spectroscopy outside the visible spectral region. Specifically, we report the use of second-harmonic generation on a frequency-modulated visible dye-laser beam to produce a frequency-modulated ultraviolet beam that is used to observe the Na 3S ? 4P absorption at 3302 A.

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http://dx.doi.org/10.1364/ol.8.000157DOI Listing

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