The idea of extending cavity quantum electrodynamics experiments to sub-wavelength sized nanomechanical systems has been recently proposed in the context of optical cavity cooling and optomechanics of deformable cavities. Here we present an experiment involving a single nanorod consisting of about 10(9) atoms precisely positioned into the confined mode of a miniature high finesse Fabry-Pérot microcavity. We show that the optical transmission of the cavity is affected not only by the static position of the nanorod but also by its vibrational fluctuation. The Brownian motion of the nanorod is resolved with a displacement sensitivity of 200 fm/square root Hz at room temperature. Besides a broad range of sensing applications, cavity-induced manipulation of optomechanical nanosystems and back-action is anticipated.
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http://dx.doi.org/10.1364/oe.17.012813 | DOI Listing |
Anal Chem
January 2025
Hefei National Laboratory, University of Science and Technology of China, Hefei 230088, China.
Detection of trace gases, such as radioactive carbon dioxide, clumped isotopes, and reactive radicals, is of great interest and poses significant challenges in various fields. Achieving both high selectivity and high sensitivity is essential in this context. We present a highly selective molecular spectroscopy method based on comb-locked, mid-infrared, cavity-enhanced, two-photon absorption.
View Article and Find Full Text PDFPhilos Trans A Math Phys Eng Sci
December 2024
Department of Physics and Astronomy, University of Exeter, Exeter, Devon EX4 4QL, UK.
Room-temperature cavity quantum electrodynamics with molecular materials in optical cavities offers exciting prospects for controlling electronic, nuclear and photonic degrees of freedom for applications in physics, chemistry and materials science. However, achieving strong coupling with molecular ensembles typically requires high molecular densities and substantial electromagnetic-field confinement. These conditions usually involve a significant degree of molecular disorder and a highly structured photonic density of states.
View Article and Find Full Text PDFVery high-average optical enhancement cavities (OECs) are being used both in fundamental and applied research. The most demanding applications require stable megawatt level average power of infrared picosecond pulses with repetition rates of several tens of MHz. Toward reaching this goal, we report on the achievement of 710 kW of stable average power in a two-mirror hemispherical optical enhancement cavity.
View Article and Find Full Text PDFWe present two distinct ultra-low frequency noise lasers at 729 nm with a fast frequency noise of 30 Hz/Hz, corresponding to a Lorentzian linewidth of 0.1 kHz. The characteristics of both lasers, which are based on different types of laser diodes, are investigated using experimental and theoretical analysis with a focus on identifying the advantages and disadvantages of each type of system.
View Article and Find Full Text PDFWe report a trace gas sensing technique of cavity-enhanced light-induced thermoelastic spectroscopy (CE-LITES) with a Fabry-Pérot (F-P) optical cavity and a high-quality-factor resonant quartz tuning fork (QTF). Pound-Drever-Hall (PDH) locking method is used to lock the laser to the optical cavity. With only a short 9-cm optical cavity (finesse, ∼1283) and a tiny commercially available standard QTF (Q-factor, ∼38910), a CE-LITES sensor for acetylene detection was developed to demonstrate this technique, achieving a minimum detection limit (MDL) of 7.
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