The transient thermal lensing in a liquid-nitrogren cooled kilohertz multipass amplifier is quantitatively measured with spatially-resolved Fourier transform spectral interferometry. A pump-probe arrangement allows the observation of a polarization-dependent non-thermal component following the fluorescence timescale: additional cooling would not suppress this residual lensing. We also observe a time-dependent thermal component that has a timescale sufficiently fast to indicate that there is cooling between shots even at a repetition rate of 1 kHz. The value of pump-induced lensing would be underestimated when performing time-averaged measurements of pump-induced phase shifts.
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http://dx.doi.org/10.1364/oe.16.018557 | DOI Listing |
Sensors (Basel)
October 2024
Dipartimento di Fisica-Politecnico di Milano and IFN-CNR, Via Gaetano Previati 1/C, 23900 Lecco, Italy.
The amplitude modulation of a pump field and the phase-sensitive detection of a pump-induced intensity change of a probe field encompass a common practice in nonlinear spectroscopies to enhance the detection sensitivity. A drawback of this approach arises when the modulation frequency is comparable to the width of the spectral feature of interest, since the presence of sidebands in the amplitude-modulated pump field provides distortion to the observed spectral lineshape. This represents a problem when accurate measurements of spectral lineshapes and line positions are pursued, as recently happened in our group with the metrology of the Q(1) line in the 1-0 band of molecular hydrogen.
View Article and Find Full Text PDFJ Chem Phys
November 2024
Molecular Spectroscopy Laboratory, RIKEN, 2-1 Hirosawa, Wako, Saitama 351-0198, Japan.
Aqueous interfaces containing organic/inorganic molecules are important in various biological, industrial, and atmospheric processes. So far, the study on the dynamics of interfacial molecules has been carried out with time-resolved vibrational sum-frequency generation (TR-VSFG) and time-resolved electronic sum-frequency generation (TR-ESFG) techniques. Although the ESFG probe is powerful for investigating interfacial photochemical dynamics of solute molecules by monitoring the electronic transition of transients or photoproducts at the interface, heterodyne detection is highly desirable for obtaining straightforward information, particularly in time-resolved measurements.
View Article and Find Full Text PDFCureus
March 2024
Cardiothoracic Anesthesiology, HCA Florida Westside Hospital, Plantation, USA.
The intra-aortic balloon pump (IABP) is a mechanical device that increases myocardial oxygen perfusion and indirectly increases cardiac output through afterload reduction. Since its inception, the IABP has been a mainstay of cardiac support devices, utilized as a temporizing measure in patients with or prone to developing cardiogenic shock that are awaiting definitive treatment. Systolic anterior motion (SAM) of the mitral valve is a well-described phenomenon that can precipitate hemodynamic collapse by obstructing the left ventricular outflow tract in a subset of patients with cardiac pathology, most notably hypertrophic obstructive cardiomyopathy (HOCM).
View Article and Find Full Text PDFUnderstanding of pump-induced lensing in laser amplifiers is essential for the optimized design of high-power lasers with high spatial quality, but there is usually incomplete knowledge of the interplay between thermal and population induced lensing mechanisms, lensing under lasing and non-lasing conditions, and transient lensing effects under pulsed operation. This paper provides quantitative insight of pump-induced lensing effects by using experimental transient pump-probe measurements in an alexandrite laser amplifier end-pumped by a short pulse pump beam with Gaussian spatial intensity distribution. Lensing results are presented showing a large difference in lensing under both non-lasing and lasing conditions and distinction of the population lens and thermal lens contributions from their different response time.
View Article and Find Full Text PDFMaterials (Basel)
March 2024
Department of Physics, Chungbuk National University, Cheongju 28644, Chungbuk, Republic of Korea.
We investigated the ultrafast dynamics of a SrRuO/BiFeO superlattice grown on a SrTiO substrate using a near infrared pump-probe technique at various temperatures. The superlattice exhibits a ferromagnetic order inherited from the SrRuO layer. The pump-induced changes in the reflectivity reveal periodic oscillations.
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