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Thermally and Base-Triggered "Debond-on-Demand" Chain-Extended Polyurethane Adhesives.
Macromolecules
January 2025
Department of Chemistry, University of Reading, Whiteknights, Reading RG6 6AD, U.K.
A series of novel chain-extended polyurethanes (CEPUs) featuring degradable sulfonyl ethyl urethane chain-extenders that permit degradation under base-triggered conditions to afford "debond-on-demand" elastomeric adhesives are reported. Exposure of the CEPUs to -butylammonium fluoride (TBAF) triggered the degradation of the sulfonyl ethyl urethane chain-extenders. Lap shear adhesion tests of the CEPUs exposed to TBAF revealed reductions in shear strength of up to 65% for both aluminum and glass substrates, from 2.
View Article and Find Full Text PDFStretchable wrinkle-structured liquid metal sandwich films enable strain-insensitive electromagnetic shielding and Joule heating.
Mater Horiz
January 2025
Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, Zhejiang province, 315201, China.
Stretchable electromagnetic interference (EMI) shields with strain-insensitive EMI shielding and Joule heating performances are highly desirable to be integrated with wearable electronics. To explore the possibility of applying geometric design in elastomeric liquid metal (LM) composites and fully investigate the influence of LM geometry on stretchable EMI shielding and Joule heating, multifunctional wrinkle-structured LM/Ecoflex sandwich films with excellent stretchability are developed. The denser LM wrinkle enables not only better electrical conduction, higher shielding effectiveness (SE) and steady-state temperature, but also enhanced strain-stable far-field/near-field shielding performance and Joule-heating capability.
View Article and Find Full Text PDFStress Relaxation Behavior of Azido Propellant Based on BAMO-THF at High Temperatures.
Materials (Basel)
December 2024
State Key Laboratory of Polymer Materials Engineering, Polymer Research Institute of Sichuan University, Chengdu 610065, China.
The azido propellant, with high energy and low signature, has been a hotpot in the field of propellants. However, the risk of low heat resistance and mechanical performance restricts their range of applications in high-energy formulations. In this study, four azido propellants based on 3,3-bis (azidomethyl) oxetane-tetrahydrofuran copolyether (BAMO-THF) have been prepared, their basic physical properties including energetic properties, internal micro-structure and true density were studied; their tensile properties, dynamic mechanical performances, were investigated, the structure-properties relationship was proposed.
View Article and Find Full Text PDFEvaluating Cost-effectiveness and Mixing Efficacy for Elastomeric and Temporary Restorative Material Using Two Mixing Tips: A SEM-EDS Analysis.
J Contemp Dent Pract
September 2024
Department of Prosthodontics and Crown & Bridge, Bharati Vidyapeeth Deemed to be University, Dental College and Hospital, Pune, Maharashtra, India, ORCID: https://orcid.org/0009-0008-7338-1699.
Aim: This study aimed to compare the mixing efficacy and cost-effectiveness of new T-mixer tips against the standard double helical tips for a light-body elastomeric impression and a temporary/interim restorative material using a scanning electron microscope (SEM) and energy-dispersive X-ray spectroscopy.
Methodology: Automixed samples ( = 16) were divided into four groups of four samples each: Samples that were mixed with Helical tip for elastomer, T-mixer tip for elastomer, Helical tip for interim restorative material, and T-mixer tip for interim restorative material. These samples were then evaluated for SEM analysis.
Poly(3-hydroxybutyrate) Modified with Thermoplastic Polyurethane and Microfibrillated Cellulose: Hydrolytic Degradation and Thermal and Mechanical Properties.
Polymers (Basel)
December 2024
Faculty of Biology, University of Bucharest, 91-95 Splaiul Independentei, 050095 Bucharest, Romania.
Blending poly(3-hydroxybutyrate) (PHB) with other polymers could be a rapid and accessible solution to overcome some of its drawbacks. In this work, PHB was modified with microfibrillated cellulose (MC) and a thermoplastic polyurethane containing biodegradable segments (PU) by two routes, using a masterbatch and by direct mixing. The PU and MC modifiers improved the thermal stability of PHB by up to 13 °C and slightly decreased its melt viscosity and crystallinity, thus improving the melt processability.
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