Antibonding ground states in InAs quantum-dot molecules.

Phys Rev Lett

Naval Research Laboratory, Washington, DC 20375, USA.

Published: January 2009

Coherent tunneling between two InAs quantum dots forms delocalized molecular states. Using magnetophotoluminescence spectroscopy we show that when holes tunnel through a thin barrier, the lowest energy molecular state has bonding orbital character. However, as the thickness of the barrier increases, the molecular ground state changes character from a bonding orbital to an antibonding orbital, confirming recent theoretical predictions. We explain how the spin-orbit interaction causes this counterintuitive reversal by using a four-band k.p model and atomistic calculations that account for strain.

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http://dx.doi.org/10.1103/PhysRevLett.102.047401DOI Listing

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