We experimentally demonstrate a strong-field coherent control mechanism that combines the advantages of photon locking (PL) and rapid adiabatic passage (RAP). Unlike earlier implementations of PL and RAP by pulse sequences or chirped pulses, we use shaped pulses generated by phase modulation of the spectrum of a femtosecond laser pulse with a generalized phase discontinuity. The novel control scenario is characterized by a high degree of robustness achieved via adiabatic preparation of a state of maximum coherence. Subsequent phase control allows for efficient switching among different target states. We investigate both properties by photoelectron spectroscopy on potassium atoms interacting with the intense shaped light field.
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http://dx.doi.org/10.1103/PhysRevLett.102.023004 | DOI Listing |
An intelligent controlled spatiotemporal mode-locked (STML) fiber laser based on a photonic lantern (PL) is proposed and experimentally demonstrated. A pair of in-house developed PLs is spliced into the cavity in a back-to-back structure. This PL-based structure functions as a mode multiplexer/demultiplexer to generate higher-order spatial modes.
View Article and Find Full Text PDFJ Am Chem Soc
January 2025
Department of Chemistry, The Hong Kong Branch of Chinese National Engineering Research Center for Tissue Restoration and Reconstruction, Division of Life Science, State Key Laboratory of Molecular Neuroscience, and Department of Chemical & Biological Engineering, The Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong 999077, China.
The two contradictory entities in nature often follow the principle of unity of opposites, leading to optimal overall performance. Particularly, aggregation-induced emission luminogens (AIEgens) with donor-acceptor (D-A) structures exhibit tunable optical properties and versatile functionalities, offering significant potential to revolutionize cancer treatment. However, trapped by low molar absorptivity (ε) owing to the distorted configurations, the ceilings of their photon-harvesting capability and the corresponding phototheranostic performance still fall short.
View Article and Find Full Text PDFSensors (Basel)
December 2024
School of Cyberspace Security, Beijing University of Post and Telecommunications, Beijing 100876, China.
As Internet of Things (IoT) technology continues to advance, there is a growing awareness of IoT security within the industry. Quantum communication technology can potentially significantly improve the communication security of IoT devices. Based on semi-quantum cryptography and utilizing single photons, this paper introduces two semi-quantum secure direct communication (SQSDC) protocols for use in smart door locks.
View Article and Find Full Text PDFAnal Chem
January 2025
Hefei National Laboratory, University of Science and Technology of China, Hefei 230088, China.
Detection of trace gases, such as radioactive carbon dioxide, clumped isotopes, and reactive radicals, is of great interest and poses significant challenges in various fields. Achieving both high selectivity and high sensitivity is essential in this context. We present a highly selective molecular spectroscopy method based on comb-locked, mid-infrared, cavity-enhanced, two-photon absorption.
View Article and Find Full Text PDFAn ultra-narrow-linewidth laser is a core device in fields such as optical atomic clocks, quantum communications, and microwave photonic oscillators. This paper reports an ultra-narrow-linewidth self-injection locked semiconductor laser, which is realized through optical feedback from a high-Q (258 million) Fabry-Perot (FP) cavity constructed with three mirrors, generating an output power of 12 mW. Employing a delay self-heterodyne method based on a signal source analyzer, the phase noise of the laser is -129 dBc/Hz at 100 kHz offset frequency, with an intrinsic linewidth of 3 mHz.
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