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Aerosol transport and associated boundary layer thermodynamics under contrasting synoptic conditions over a semiarid site.

Sci Total Environ

January 2025

Department of Geosciences, Atmospheric Science Division, Texas Tech University, Lubbock, TX, USA; National Wind Institute, Texas Tech University, Lubbock, TX, USA. Electronic address:

Understanding the kinematics of aerosol horizontal transport and vertical mixing near the surface, within the atmospheric boundary layer (ABL), and in the overlying free troposphere (FT) is critical for various applications, including air quality and weather forecasting, aviation, road safety, and dispersion modeling. Empirical evidence of aerosol mixing processes within the ABL during synoptic-scale events over arid and semiarid regions (i.e.

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Aerosol particles in the PM fraction considerably influence the climate-related effects of aerosols and impact human health despite representing very variable fractions of the total aerosol mass concentration. Aerosol optical measurement techniques (aerosol light scattering) may not be sufficiently effective for detecting all particles in the PM fraction, particularly regarding number concentration. The present study investigates temporal variations of aerosol light scattering properties and particle number concentration (PNC) at different size modes in the PM fraction at the atmospheric site ATOLL (The Atmospheric Observations in Lille), Northern France from January 2018 to February 2023.

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A detailed protocol for measuring the complex forward-scattering amplitude S(0°) of single particles, the Complex Amplitude Sensing version 1 (CAS-v1), has recently been developed and used for characterizing environmental particles. However, interpretations of the S(0°) data need a priori assumptions on the particle's shape, and applications of the method have mostly been limited to the particles suspended in liquids. Here, we thoroughly upgrade the CAS technique to perform quality-controlled S(0°) measurements at two independent polarizations for particles suspended in gases and liquids.

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Ex-situ Raman spectroscopy is a well-established method for the structural characterization of soot but necessitates a sampling step before analysis is made. This work studied the potential to perform Raman spectroscopic measurements of soot directly in the combustion exhaust gases, i.e.

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Microplastic pollution presents a serious risk to marine ecosystems worldwide, with West Africa being especially susceptible. This study sought to identify the key factors driving microplastic dynamics in the region. Using NASA's Giovanni system, we analyzed environmental data from 2019 to 2024.

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