Coherent acoustic phonons are generated at terahertz frequencies when semiconductor quantum-well nanostructures are illuminated by femtosecond laser pulses. These phonons-also known as nanoacoustic waves-typically have wavelengths of tens of nanometres, which could prove useful in applications such as non-invasive ultrasonic imaging and sound amplification by the stimulated emission of radiation. However, optical diffraction effects mean that the nanoacoustic waves are produced with spot sizes on the micrometre scale. Near-field optical techniques can produce waves with smaller spot sizes, but they only work near surfaces. Here, we show that a far-field optical technique--which suffers no such restrictions--can be used to spatially manipulate the phonon generation process so that nanoacoustic waves are emitted with lateral dimensions that are much smaller than the laser wavelength. We demonstrate that nanoacoustic waves with wavelengths and spot sizes of the order of 10 nm and 100 nm, respectively, can be generated and detected.
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http://dx.doi.org/10.1038/nnano.2007.319 | DOI Listing |
Int J Nanomedicine
December 2024
Department of Abdominal Ultrasound, The Affiliated Hospital of Qingdao University, Qingdao, People's Republic of China.
Sonodynamic therapy (SDT) utilizes specific sound waves to activate sonosensitizers, generating localized biological effects to eliminate tumor cells. With advancements in nanomedicine, the application of nano-acoustic sensitizers has significantly advanced the development of SDT. BaTiO (BTO), an inorganic nano-acoustic sensitizer, possesses light refraction characteristics and a high dielectric constant, and can generate an electric field under ultrasound (US) stimulation.
View Article and Find Full Text PDFNat Commun
June 2022
Key Laboratory of Mesoscopic Chemistry of MOE, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing, 210023, China.
Sensitive detection of local acoustic vibrations at the nanometer scale has promising potential applications involving miniaturized devices in many areas, such as geological exploration, military reconnaissance, and ultrasound imaging. However, sensitive detection of weak acoustic signals with high spatial resolution at room temperature has become a major challenge. Here, we report a nanometer-scale system for acoustic detection with a single molecule as a probe based on minute variations of its distance to the surface of a plasmonic gold nanorod.
View Article and Find Full Text PDFPhotoacoustics
September 2021
Laboratoire d'Acoustique de l'Université du Mans (LAUM), UMR 6613, Institut d'Acoustique - Graduate School (IA-GS), CNRS, Le Mans Université, France.
Non-invasive fast imaging of grain microstructure of polycrystalline ceria with sub-micrometric spatial resolution is performed via time-domain Brillouin scattering. The propagation of a nanoacoustic pulse is monitored down to 8 μm deep in a 30 × 30 μm area. Grains boundaries are reconstructed in three-dimensions via a two-step processing method, relying on the wavelet synchro-squeezed transform and the alphashape algorithm.
View Article and Find Full Text PDFSmall
April 2020
Pillar of Engineering Product Development, Singapore University of Technology and Design, Singapore, 487372, Singapore.
Nanoacoustic fields are a promising method for particle actuation at the nanoscale, though THz frequencies are typically required to create nanoscale wavelengths. In this work, the generation of robust nanoscale force gradients is demonstrated using MHz driving frequencies via acoustic-structure interactions. A structured elastic layer at the interface between a microfluidic channel and a traveling surface acoustic wave (SAW) device results in submicron acoustic traps, each of which can trap individual submicron particles.
View Article and Find Full Text PDFSci Rep
September 2014
1] Department of Electrical Engineering and Graduate Institute of Photonics and Optoelectronics, National Taiwan University, Taipei 10617, Taiwan [2] Institute of Physics and Research Center for Applied Science, Academia Sinica, Taipei 115, Taiwan [3] Molecular Imaging Center, National Taiwan University, Taipei 10617, Taiwan [4] Graduate Institute of Biomedical Electronics and Bioinformatics and Center for Optoelectronics Medicine, National Taiwan University, Taipei 10617, Taiwan.
Despite the numerous devoted studies, water at solid interfaces remains puzzling. An ongoing debate concerns the nature of interfacial water at a hydrophilic surface, whether it is more solid-like, ice-like, or liquid-like. To answer this question, a complete picture of the distribution of the water molecule structure and molecular interactions has to be obtained in a non-invasive way and on an ultrafast time scale.
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