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Silver-purine MOFs for high-performance multi-terminal neuromorphic memory.
Mater Horiz
January 2025
School of Chemical Sciences, National Institute of Science Education and Research (NISER), An OCC of HBNI, Bhubaneswar, 752050, Odisha, India.
Neuromorphic and fully analog in-memory computations are promising for handling vast amounts of data with minimal energy consumption. We have synthesized and studied a series of homo-bimetallic silver purine MOFs (1D and 2D) having direct metal-metal bonding. The N7-derivatized purine ligands are designed to form bi-metallic complexes under ambient conditions, extending to a 1D or 2D metal-organic framework.
View Article and Find Full Text PDFA Rapid Methodology to Obtain Silver Selenide thin Films with Highly Enhanced Thermoelectric Performance.
Small
January 2025
Departamentde Física Aplicada-IDF. Univérsitat Politécnica de Valéncia, Camí de Vera s/n, Valencia, 46022, Spain.
Metal chalcogenides have been extensively studied for thermoelectric applications. Among other metal chalcogenides, silver selenide (AgSe) is considered one of the most promising n-type semiconducting materials for thermoelectric applications due to its low band gap value, Seebeck coefficient, and superior power factor (PF) rendered at room temperature. However, one of the main drawbacks of using AgSe as a thermoelectric material on a large scale is the time-consuming physical methods to obtain them, and the need for high vacuum synthesis conditions as well as high-cost.
View Article and Find Full Text PDFMicrofluidic Thread-Based Analytical Platform for Reaction Screening Enabled by In Situ Thread Spray Mass Spectrometry.
Anal Chem
January 2025
Department of Chemistry and Biochemistry, The Ohio State University, Columbus, Ohio 43210, United States.
This study describes a microfluidic thread-based analytical device (μTAD) capable of in situ mass spectrometric analysis for continuous flow reaction monitoring. Organic reaction screening is foundational to drug discovery. Microfluidic devices are of special interest here because they provide continuous reaction monitoring with advantages such as the use of smaller reagent volumes and short analysis times.
View Article and Find Full Text PDFConvergent Total Synthesis of Ixabepilone and Its Analogues Enabled by Highly Efficient Asymmetric Hydrogenations.
Chemistry
December 2024
Southern University of Science and Technology, Chemistry, 1088 Xueyuan Avenue, 518055, Shenzhen, CHINA.
The convergent total synthesis of ixabepilone and its analogues in a 13-step longest linear sequence is reported. The crucial chiral centers at challenging C3-O, C8-C and C15-N positions on the scaffold of the ixabepilone were installed via highly efficient asymmetric hydrogenations (up to 95% yield and up to 99% e.e.
View Article and Find Full Text PDFArchitecting highly hydratable and permeable dense Janus membrane for rapid and robust membrane distillation desalination.
Water Res
December 2024
School of Environmental Science and Engineering, Shanghai Jiao Tong University, 800 Dongchuan Road, Shanghai 200240, Shanghai, PR China. Electronic address:
Dense Janus membranes (JMs) are potential candidates in hypersaline wastewater treatments for membrane distillation (MD). However, dense surface layers generally add obvious membrane mass transfer resistance, limiting its practical application. In this study, a novel dense JM was facilely developed by controlled interfacial polymerization utilizing a phosphonium functional monomer (THPC) on hydrophilic polyvinylidene fluoride (PVDF) substrate.
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