The dynamics of charge carriers close to the Mott transition is explored theoretically and experimentally in the quasi-two-dimensional organic charge-transfer salt, kappa-(BEDT-TTF)_(2)Cu[N(CN)_(2)]Br_(x)Cl_(1-x), with varying Br content. The frequency dependence of the conductivity deviates significantly from simple Drude model behavior: there is a strong redistribution of spectral weight as the Mott transition is approached and with temperature. The effective mass of the quasiparticles increases considerably when coming close to the insulating phase. A dynamical mean-field-theory treatment of the relevant Hubbard model gives good quantitative description of experimental data.
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| http://dx.doi.org/10.1103/PhysRevLett.100.086404 | DOI Listing |
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