Simple method of detecting ferroelectric domains with non-phase-matched second-harmonic generation.

Appl Opt

Department of Lasers, Optics, and Remote Sensing, Sandia National Laboratories, Albuquerque, New Mexico 87185-1423, USA.

Published: May 1998

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We demonstrate a new method of detecting the presence of ferroelectric domains based on non-phase-matched second-harmonic generation. If a domain boundary is tilted relative to the input and output faces of the crystal, the far-field second-harmonic light consists of multiple beams, in contrast to the single beam generated in a single-domain crystal. The angular separation of the beams provides a measure of the tilt of the domain wall if the refractive-index difference n(2omega)-n(omega) is known.

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http://dx.doi.org/10.1364/ao.37.003311DOI Listing

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