We address the quantum transition of a spin-1/2 antiferromagnetic Kondo lattice model with an easy-axis anisotropy using the extended dynamical mean field theory. We derive results in real frequency by using the bosonic numerical renormalization group (BNRG) method and compare them with quantum Monte Carlo results in Matsubara frequency. The BNRG results show a logarithmic divergence in the critical local spin susceptibility, signaling a destruction of Kondo screening. The T=0 transition is consistent with being second order. The BNRG results also display some subtle features; we identify their origin and suggest means for further microscopic studies.
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http://dx.doi.org/10.1103/PhysRevLett.99.227204 | DOI Listing |
Nat Commun
December 2024
Department of Physics, Washington University in St. Louis, St. Louis, MO, 63130, USA.
Proc Natl Acad Sci U S A
December 2024
Stanford Institute for Materials and Energy Sciences, Stanford Linear Accelerator Center (SLAC) National Accelerator Laboratory, Menlo Park, CA 94025.
Recent experiments suggest a new paradigm toward novel colossal magnetoresistance (CMR) in a family of materials EuM[Formula: see text]X[Formula: see text] (M [Formula: see text] Cd, In, Zn; X [Formula: see text] P, As), distinct from the traditional avenues involving Kondo-Ruderman-Kittel-Kasuya-Yosida crossovers, magnetic phase transitions with structural distortions, or topological phase transitions. Here, we use angle-resolved photoemission spectroscopy and density functional theory calculations to explore their origin, particularly focusing on EuCd[Formula: see text]P[Formula: see text]. While the low-energy spectral weight royally tracks that of the resistivity anomaly near the temperature with maximum magnetoresistance ([Formula: see text]) as expected from transport-spectroscopy correspondence, the spectra are completely incoherent and strongly suppressed with no hint of a Landau quasiparticle.
View Article and Find Full Text PDFNat Commun
November 2024
Departamento Física de la Materia Condensada, Universidad Autónoma de Madrid, Cantoblanco, 28049, Madrid, Spain.
The prominent role of electron-electron interactions in two-dimensional (2D) materials is at the origin of a great variety of fermionic correlated states reported in the literature. Artificial van der Waals heterostructures comprising single layers of highly correlated insulators allow one to explore the effect of the subtle interlayer interaction in the way electrons interact. We study the temperature dependence of the electronic properties of a van der Waals heterostructure composed of a single-layer Mott insulator lying on a metallic substrate by performing quasi-particle interference (QPI) maps.
View Article and Find Full Text PDFAdv Mater
November 2024
Department of Physics, Washington University in St. Louis, St. Louis, MO, 63130, USA.
Since the initial discovery of 2D van der Waals (vdW) materials, significant effort has been made to incorporate the three properties of magnetism, band structure topology, and strong electron correlations-to leverage emergent quantum phenomena and expand their potential applications. However, the discovery of a single vdW material that intrinsically hosts all three ingredients has remained an outstanding challenge. Here, the discovery of a Kondo-interacting topological antiferromagnet is reported in the vdW 5f electron system UOTe.
View Article and Find Full Text PDFJ Phys Condens Matter
December 2024
Theoretical Division, Los Alamos National Laboratory, Los Alamos, NM 87545, United States of America.
Time-resolved ultrafast spectroscopy has emerged as a promising tool to dynamically induce and manipulate non-trivial electronic states of matter out-of-equilibrium. Here we theoretically investigate light pulse driven dynamics in a Kondo lattice system close to quantum criticality. Based on a time-dependent auxiliary fermion mean-field calculation we show that light can dehybridize the local Kondo screening and induce oscillating magnetic order out of a previously paramagnetic state.
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