The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multiheterodyne spectroscopy. We measure the absorption and phase shift experienced by each of 155 000 individual frequency-comb lines, spaced by 100 MHz and spanning from 1495 to 1620 nm, after passing through hydrogen cyanide gas. The measured phase spectrum agrees with the Kramers-Kronig transformation of the absorption spectrum. This technique can provide a full complex spectrum rapidly, over wide bandwidths, and with hertz-level accuracy.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1103/PhysRevLett.100.013902 | DOI Listing |
Photoacoustics
August 2024
State Key Laboratory of Quantum Optics and Quantum Optics Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan 030006, China.
Dual-comb photoacoustic spectroscopy (DC-PAS) advances spectral measurements by offering high-sensitivity and compact size in a wavelength-independent manner. Here, we present a novel cantilever-enhanced DC-PAS scheme, employing a high-sensitivity fiber-optic acoustic sensor based on an optical cantilever and a non-resonant photoacoustic cell (PAC) featuring a flat-response characteristic. The dual comb is down-converted to the audio frequency range, and the resulting multiheterodyne sound waves from the photoacoustic effect, are mapped into the response frequency region of the optical cantilever microphone.
View Article and Find Full Text PDFLight Sci Appl
March 2024
State Key Laboratory of Quantum Optics and Quantum Optics Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan, 030006, China.
The extension of dual-comb spectroscopy (DCS) to all wavelengths of light along with its ability to provide ultra-large dynamic range and ultra-high spectral resolution, renders it extremely useful for a diverse array of applications in physics, chemistry, atmospheric science, space science, as well as medical applications. In this work, we report on an innovative technique of quartz-enhanced multiheterodyne resonant photoacoustic spectroscopy (QEMR-PAS), in which the beat frequency response from a dual comb is frequency down-converted into the audio frequency domain. In this way, gas molecules act as an optical-acoustic converter through the photoacoustic effect, generating heterodyne sound waves.
View Article and Find Full Text PDFLight Sci Appl
January 2024
Department of Mechanical and Automation Engineering, The Chinese University of Hong Kong, New Territories, Hong Kong SAR, China.
Photoacoustic dual-comb spectroscopy (DCS), converting spectral information in the optical frequency domain to the audio frequency domain via multi-heterodyne beating, enables background-free spectral measurements with high resolution and broad bandwidth. However, the detection sensitivity remains limited due to the low power of individual comb lines and the lack of broadband acoustic resonators. Here, we develop cavity-enhanced photoacoustic DCS, which overcomes these limitations by using a high-finesse optical cavity for the power amplification of dual-frequency combs and a broadband acoustic resonator with a flat-top frequency response.
View Article and Find Full Text PDFAn electro-optic dual-comb system based on chirped-pulse waveforms is used to simultaneously acquire temporally magnified rapid passage signals and normal spectral line shapes from the back-transformation to the time domain. Multi-heterodyne terahertz (THz) wave generation and detection is performed with the difference frequency mixing of two free-running lasers. The method is used to obtain THz spectra of formic acid in the 10 cm to 20 cm (300 GHz-600 GHz) region over a range of pressures.
View Article and Find Full Text PDFSensors (Basel)
May 2022
Sensors and Instrumentation Techniques Research Group, Electronics Technology Department, University Carlos III of Madrid, 28911 Leganes, Spain.
Dual-comb multiheterodyne spectroscopy is a well-established technology for the highly sensitive real-time detection and measurement of the optical spectra of samples, including gases and fiber sensors. However, a common drawback of dual-comb spectroscopy is the need for a broadband amplitude-resolved absorption or reflection measurement, which increases the complexity of the dual comb and requires the precise calibration of the optical detection. In the present study, we present an alternative dispersion-based approach applied to fiber Bragg grating sensors in which the dual comb is compacted by a single dual-drive-unit optical modulator, and the fiber sensor is part of a dispersion interferometer.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!