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Convergent-beam attosecond x-ray crystallography.
Struct Dyn
January 2025
Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607 Hamburg, Germany.
Sub-ångström spatial resolution of electron density coupled with sub-femtosecond to few-femtosecond temporal resolution is required to directly observe the dynamics of the electronic structure of a molecule after photoinitiation or some other ultrafast perturbation, such as by soft X-rays. Meeting this challenge, pushing the field of quantum crystallography to attosecond timescales, would bring insights into how the electronic and nuclear degrees of freedom couple, enable the study of quantum coherences involved in molecular dynamics, and ultimately enable these dynamics to be controlled. Here, we propose to reach this realm by employing convergent-beam x-ray crystallography with high-power attosecond pulses from a hard-x-ray free-electron laser.
View Article and Find Full Text PDFIn this Letter, we report an ultraflat high-power supercontinuum (SC) based on a low-loss short-length fluorotellurite fiber. A novel high-peak power dual-Raman soliton femtosecond laser is used as a pump source, which effectively extends the mid-infrared SC spectral range and enhances the flatness of the SC. Finally, we obtained a 10.
View Article and Find Full Text PDFDynamic transverse mode instability (TMI) has become one of the primary limitations for power scaling of high-power fiber lasers. Experimental evidence has shown that static mode degradation can suppress the dynamic TMI effect. This study reveals the physical mechanisms behind the mitigation of dynamic TMI in two-mode fiber lasers through static mode degradation.
View Article and Find Full Text PDFA 1645 nm end-pumped dual-channel Er:YAG vector laser that could generate two cylindrical vector (CV) beams simultaneously with different polarization orders is demonstrated. The laser is designed in a two-arm structure, wherein each arm places a q-plate (QP) to introduce intra-cavity spin-orbital angular momentum conversion, leading to the oscillation of two various CV modes in two arms, and finally output along two directions, respectively. The favorable experimental results illustrate high power stability and polarization mode purity.
View Article and Find Full Text PDFThe control of temporal noise of the pump could add an additional degree of freedom to manipulate the spectrum of continuous-wave (CW) pumped SC generation. In this paper, we experimentally tailor the CW-pumped supercontinuum (SC) generation in a cascaded Raman random fiber laser (CRRFL) based on a 1 µm pump with tunable temporal dynamics. The pump is based on a spectrally filtered ytterbium-doped random fiber laser (YRFL) seed laser, which can be amplified to a 10 W level with the tunable temporal noise.
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