An experimental technique based on coherent one-dimensional hyper-Raman-resonant four-wave mixing in broad cylindrically focused light beams has been developed for line-by-line imaging of spatial distribution of excited atoms in a low-temperature plasma of optical breakdown. The technique was applied to map excited lead atoms in a low-temperature laser-produced plasma.
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http://dx.doi.org/10.1364/ol.24.000478 | DOI Listing |
ACS Photonics
January 2025
Cardiff University School of Physics and Astronomy, The Parade, Cardiff CF24 3AA, United Kingdom.
The field of chiral nanoparticles is rapidly expanding, yet measuring the chirality of single nano-objects remains a challenging endeavor. Here, we report a technique to detect chiro-optical effects in single plasmonic nanoparticles by means of phase-sensitive polarization-resolved four-wave mixing interferometric microscopy. Beyond conventional circular dichroism, the method is sensitive to the particle polarizability, in amplitude and phase.
View Article and Find Full Text PDFACS Photonics
January 2025
Electrical and Computer Engineering Department, University of California, Santa Barbara, California 93106, United States.
Correlated photon-pair sources are key components for quantum computing, networking, synchronization, and sensing applications. Integrated photonics has enabled chip-scale sources using nonlinear processes, producing high-rate time-energy and polarization entanglement at telecom wavelengths with sub-100 microwatt pump power. Many quantum systems operate in the visible or near-infrared ranges, necessitating visible-telecom entangled-pair sources for connecting remote systems via entanglement swapping and teleportation.
View Article and Find Full Text PDFIn this study, we investigated in detail the regulation mechanism of electron transfer under laser-induced breakdown (LIB) on weak O-D stimulated Raman scattering (SRS) in DMSO-DO solutions. Significantly, the Raman activity of O-D vibrations was greatly enhanced by two orders of magnitude due to electron transfer in DMSO molecules. Density functional theory (DFT) calculations showed that the O-D Raman activity was significantly enhanced in the DMSO-DO dimer compared to the DO dimer.
View Article and Find Full Text PDFLarge-scale quantum photonic circuits require integrating multiple single-photon sources, which are typically based on spontaneous four-wave mixing (SFWM) in spiral waveguides or microring resonators (MRRs). Photons can be generated in both clockwise (CW) and counterclockwise (CCW) orientations from a single source in a Sagnac configuration, showing promise for improving scalability. In this work, we propose a fully integrable scheme for bidirectional creation and usage of single photons.
View Article and Find Full Text PDFLight Sci Appl
January 2025
Department of Electronics and Nanoengineering, Aalto University, Espoo, Finland.
Coherent broadband light generation has attracted massive attention due to its numerous applications ranging from metrology, sensing, and imaging to communication. In general, spectral broadening is realized via third-order and higher-order nonlinear optical processes (e.g.
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