Inelastic neutron scattering experiments have been performed on the archetype compound YbB(12), using neutron polarization analysis to separate the magnetic signal from the phonon background. With decreasing temperature, components characteristic for a single-site spin-fluctuation dynamics are suppressed, giving place to specific, strongly Q-dependent, low-energy excitations near the spin-gap edge. This crossover is discussed in terms of a simple crystal-field description of the incoherent high-temperature state and a predominantly local mechanism for the formation of the low-temperature singlet ground state.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1103/PhysRevLett.99.137204 | DOI Listing |
Angew Chem Int Ed Engl
January 2025
Department of Chemistry, School of Green Chemistry and Engineering, The University of Toledo, Toledo, Ohio, 43606, United States.
The chemistry of electrons in actinide complexes and materials is still poorly understood and represents a serious challenge and opportunity for experiment and theory. The study of the electron density distribution of the ground state of such systems through X-ray diffraction represents a unique opportunity to quantitatively investigate different chemical bonding interactions at once, but was considered "almost impossible" on heavy-atom systems, until very recently. Here, we present a combined experimental and theoretical investigation of the electron density distribution in UCl_ crystals and comparison with the previously reported spin density distribution from polarized neutron diffraction.
View Article and Find Full Text PDFNatl Sci Rev
August 2024
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
The magnetic correlations at the superconductor/ferromagnet (S/F) interfaces play a crucial role in realizing dissipation-less spin-based logic and memory technologies, such as triplet-supercurrent spin-valves and 'π' Josephson junctions. Here we report the observation of an induced large magnetic moment at high-quality nitride S/F interfaces. Using polarized neutron reflectometry and DC SQUID measurements, we quantitatively determined the magnetization profile of the S/F bilayer and confirmed that the induced magnetic moment in the adjacent superconductor only exists below .
View Article and Find Full Text PDFAdv Sci (Weinh)
September 2024
Rutger Center for Emergent Materials and Department of Physics and Astronomy, Rutgers University, Piscataway, NJ, 08854, USA.
Ferro-rotational (FR) materials, renowned for their distinctive material functionalities, present challenges in the growth of homo-FR crystals (i.e., single FR domain).
View Article and Find Full Text PDFRev Sci Instrum
June 2024
Helmholtz Centre Berlin for Materials and Energy, D-14109 Berlin, Germany.
This work describes the implementation of polarized neutron imaging capabilities at the neutron and x-ray tomograph (NeXT) imaging station of the Institut Laue Langevin. This development enhances the capacity of this instrument to study advanced magnetic materials, which are crucial in a variety of engineering applications. Here, the feasibility of polarized neutron imaging at NeXT is demonstrated by visualizing the magnetic field generated by a simple bar magnet.
View Article and Find Full Text PDFJ Chem Phys
February 2024
European Synchrotron Radiation Facility, 71, Avenue des Martyrs, CS40220, F-38043 Grenoble CEDEX 9, France.
Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!