Low field laser ionization of argon clusters: the remarkable fragmentation dynamics of doubly ionized clusters.

Phys Rev Lett

Laboratoire Francis Perrin, CEA/DSM/DRECAM/SPAM-CNRS URA 2453, C.E.A. Saclay, F-91191 Gif-sur-Yvette cedex, France.

Published: September 2007

We have investigated the fission following a Coulomb explosion in argon clusters (up to Ar800) irradiated by a femtosecond infrared laser with moderate intensity IL approximately 10(13) W cm(-2). We report the a priori surprising observation of well-defined velocity distributions of the ionized fragments Ar+n<50. This is interpreted by the formation of a valence shell excited charged ion, followed by relaxation, charge transfer by autoionizing collision at very short distance, and asymmetric fission.

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http://dx.doi.org/10.1103/PhysRevLett.99.103401DOI Listing

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