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The Quantum Information Science Challenge for Chemistry.
J Phys Chem Lett
January 2025
Department of Chemistry, College of Science, University of Nevada, Reno, Nevada 89557, United States.
We discuss the goals and the need for quantum information science (QIS) in chemistry. It is important to identify concretely how QIS matters to chemistry, and we articulate some of the most pressing and interesting research questions at the interface between chemistry and QIS, that is, "chemistry-centric" research questions relevant to QIS. We propose in what ways and in what new directions the field should innovate, in particular where a chemical perspective is essential.
View Article and Find Full Text PDFDeep Thermalization in Gaussian Continuous-Variable Quantum Systems.
Phys Rev Lett
December 2024
National University of Singapore, Department of Physics, Singapore 117551.
We uncover emergent universality arising in the equilibration dynamics of multimode continuous-variable systems. Specifically, we study the ensemble of pure states supported on a small subsystem of a few modes, generated by Gaussian measurements on the remaining modes of a globally pure bosonic Gaussian state. We find that beginning from highly entangled, complex global states, such as random Gaussian states and product squeezed states coupled via a deep array of linear optical elements, the induced ensemble attains a universal form, independent of the choice of measurement basis: it is composed of unsqueezed coherent states whose displacements are distributed normally and isotropically, with variance depending on only the particle-number density of the system.
View Article and Find Full Text PDFQuantum Analog of Landau-Lifshitz-Gilbert Dynamics.
Phys Rev Lett
December 2024
Uppsala University, Department of Physics and Astronomy, Box 516, SE-751 20 Uppsala, Sweden.
The Landau-Lifshitz-Gilbert (LLG) and Landau-Lifshitz (LL) equations play an essential role for describing the dynamics of magnetization in solids. While a quantum analog of the LL dynamics has been proposed in [Phys. Rev.
View Article and Find Full Text PDFUnified Variational Approach Description of Ground-State Phases of the Two-Dimensional Electron Gas.
Phys Rev Lett
December 2024
Flatiron Institute, Center for Computational Quantum Physics, New York, New York 10010, USA.
The two-dimensional electron gas (2DEG) is a fundamental model, which is drawing increasing interest because of recent advances in experimental and theoretical studies of 2D materials. Current understanding of the ground state of the 2DEG relies on quantum Monte Carlo calculations, based on variational comparisons of different Ansätze for different phases. We use a single variational ansatz, a general backflow-type wave function using a message-passing neural quantum state architecture, for a unified description across the entire density range.
View Article and Find Full Text PDFQuantum Thermodynamic Derivation of the Energy Resolution Limit in Magnetometry.
Phys Rev Lett
December 2024
University of Crete, Department of Physics, Heraklion 70013, Greece.
It was recently demonstrated that a multitude of realizations of several magnetic sensing technologies satisfy the energy resolution limit, which connects a quantity composed by the variance of the magnetic field estimate, the sensor volume and the measurement time, and having units of action, with ℏ. A first-principles derivation of this limit is still elusive. We here present such a derivation based on quantum thermodynamic arguments.
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