Treatment of seven tetracycline classes of antibiotic (TAs) from raw waters (synthetic and river) was evaluated using coagulation and granular activated carbon (GAC) filtration in this study. Both coagulation and GAC filtration were effective for removal of TAs, and the removal efficiency depended on the type of TAs. GAC filtration was relatively more effective for removal of tetracycline (TC), doxycycline-hyclate (DXC), and chlortetracycline-HCl (CTC), which were difficult to remove by coagulation. It was speculated that TAs would be removed through the charge neutralization and sweep coagulation when poly-aluminum chloride (PACl) was added into the raw waters. The charge neutralization of zwitterionic or negative TAs by cationic Al (III) species drove removal of TAs from the synthetic water. When sufficient alkalinity was available (river water), aluminum hydroxide precipitates were formed. TAs could be removed by being enmeshed into or adsorbed onto the precipitates when PACl was added to the river water.
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http://dx.doi.org/10.1016/j.jhazmat.2007.05.059 | DOI Listing |
Chemosphere
November 2024
Department of Civil, Geological and Mining Engineering, Polytechnique Montréal, Montréal, Quebec, Canada.
J Hazard Mater
December 2024
Department of Civil and Environmental Engineering, Norwegian University of Science and Technology (NTNU), S. P. Andersens veg 5, 7031 Trondheim, Norway. Electronic address:
Tunnel wash water (TWW) contains high levels of trace elements and organic micropollutants, especially in the dissolved fraction. Discharge poses significant environmental risks. This field study aimed at improving conventional sedimentation treatment by addition of novel secondary treatments: bag filtration, ceramic microfiltration, or granular activated carbon (GAC) filtration.
View Article and Find Full Text PDFWater Res
January 2025
Key Laboratory of Drinking Water Science and Technology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China; University of Chinese Academy of Sciences, Beijing 100049, China.
The proliferation of pathogenic bacteria and antibiotic resistance genes (ARGs) in the biofilm of drinking water distribution pipes poses a serious threat to human health. This work adopted 15 polyethylene (PE) pipes to study the co-selective effect of dissolved organic matter (DOM) and chlorine on the bacterial community and their antibiotic resistance in biofilm. The results indicated that ozone and granular activated carbon (O-GAC) filtration effectively removed lignins and proteins from DOM, and chlorine disinfection eliminated carbohydrate and unsaturated hydrocarbons, which both contributed to the inhibition of bacterial growth and biofilm formation.
View Article and Find Full Text PDFWater Res
January 2025
Department of Civil & Environmental Engineering, University of Waterloo, Waterloo, Ontario, N2L 3G1, Canada.
This study investigated the influence of filter media characteristics on manganese (Mn) removal in groundwater biofilters during the start-up phase. Six pilot scale biofilters containing three different granular activated carbons (GAC), two anthracite, and one sand media were run for 133 days to examine their Mn removal performance at a drinking water utility, while also monitoring ATP and bacterial growth as indicators of biological activity. Key findings demonstrate the critical role of media characteristics, especially for GAC media.
View Article and Find Full Text PDFSci Total Environ
December 2024
Cranfield University, Cranfield MK43 0AL, UK. Electronic address:
In a well-functioning slow sand filter (SSF), dissolved oxygen (DO) is crucial for enabling aerobic processes and microbiota growth. Given that DO supply is predominantly via the feed water, flow pauses (e.g.
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