The dynamics of vibrational wave packets excited in Na2 dimers in the triplet ground and excited states is investigated by means of helium nanodroplet isolation (HENDI) combined with femtosecond pump-probe spectroscopy. Different pathways in the employed resonant multiphoton ionization scheme are identified. Within the precision of the method, the wave packet dynamics appears to be unperturbed by the helium droplet environment.
Download full-text PDF |
Source |
|---|---|
| http://dx.doi.org/10.1021/jp070893i | DOI Listing |
Publication Analysis
Top Keywords
Similar Publications
Elastic Wave Packets Crossing a Space-Time Interface.
Phys Rev Lett
December 2024
Institut Langevin, ESPCI Paris, Université PSL, CNRS, 75005 Paris, France.
The interaction between waves and evolving media challenges traditional conservation laws. We experimentally investigate the behavior of elastic wave packets crossing a moving interface that separates two media with distinct propagation properties, observing the noninvariance of wavelength and frequency. Our experimental setup employs an elastic strip whose local stretching can be dynamically altered by pulling one end at a constant velocity.
View Article and Find Full Text PDFUnambiguous Detection of High-Energy Vortex States via the Superkick Effect.
Phys Rev Lett
December 2024
Sun Yat-sen University, School of Physics and Astronomy, Zhuhai 519082, China.
Vortex states of photons, electrons, and other particles are freely propagating wave packets with helicoidal wave fronts winding around the axis of a phase vortex. A particle prepared in a vortex state carries a nonzero orbital angular momentum projection on the propagation direction, a quantum number that has never been exploited in experimental particle and nuclear physics. Low-energy vortex photons, electrons, neutrons, and helium atoms have been demonstrated in experiment and found numerous applications, and there exist proposals of boosting them to higher energies.
View Article and Find Full Text PDFUse of Resonant Acoustic Fields as Atmospheric-Pressure Ion Gates.
Anal Chem
January 2025
Department of Chemistry and Chemical Biology, Rensselaer Polytechnic Institute, Troy, New York 12180, United States.
Ion optics are crucial for spectrometric methods such as mass spectrometry (MS) and ion mobility spectrometry (IMS). Among the wide selection of ion optics, temporal ion gates are of particular importance for time-of-flight MS (TOF-MS) and drift-tube IMS. Commonly implemented as electrostatic ion gates, these optics offer a rapid, efficient means to block ion beams and form discrete ion packets for subsequent analysis.
View Article and Find Full Text PDFThe space-time wave packet (STWP) is a type of pulsed optical field, exhibiting distinctive characteristics, including the capacity to propagate without diffraction or dispersion and to have arbitrary group velocities. However, the intensity of the STWP is constrained by the low damage threshold of some indispensable optical elements like the spatial light modulator (SLM). While optical parametric amplification (OPA) has been proposed for amplifying STWPs, spatio-temporal (ST) characteristics of amplified STWPs remain significantly unexplored.
View Article and Find Full Text PDFA transversely isotropic diode-pumped solid-state laser is used to obtain an orthogonally dual-polarization nonplanar circular mode (NCM) under off-axis pumping in the strictly degenerate cavity. Each polarized component of the NCM outside the cavity is revealed to be individually localized on the ray orbits forming a nonplanar surface, in which the transverse patterns display multiple spots well positioned on a circular structure. An analytical representation is established to explore polarization-resolved components of the NCM by utilizing the Gaussian wave packet to directly correlate with geometrical rays.
View Article and Find Full Text PDFWant AI Summaries of new PubMed Abstracts delivered to your In-box?
Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!