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Photodissociation of vibrationally excited SH and SD radicals at 288 and 291 nm: the S(1D2) channel. | LitMetric
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Photodissociation of vibrationally excited SH and SD radicals at 288 and 291 nm: the S(1D2) channel.

Liesbeth M C Janssen Mark P J van der Loo Gerrit C Groenenboom Shiou-Min Wu Dragana C Radenović André J A van Roij Ivan Anton Garcia David H Parker

J Chem Phys

Theoretical Chemistry, Institute for Molecules and Materials (IMM), Radboud University Nijmegen, Toernooiveld 1, 6525 ED Nijmegen, The Netherlands.

Published: March 2007

Ultraviolet photodissociation of SH (X 2Pi, upsilon"=2-7) and SD (X 2Pi, upsilon"=3-7) has been studied at 288 and 291 nm, using the velocity map imaging technique to probe the angular and speed distributions of the S(1D2) products. Photodissociation cross sections for the A 2Sigma+<--X 2Pi(upsilon") and 2Delta<--X 2Pi(upsilon") transitions have been obtained by ab initio calculations at the CASSCF-MRSDCI/aug-cc-pV5Z level of theory. Both the experimental and theoretical results show that SH/SD photodissociation from X 2Pi (upsilon"

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http://dx.doi.org/10.1063/1.2646522DOI Listing

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