Despite the availability of a spin Hamiltonian for the Gd(3)Ga(5)O(12) garnet (GGG) for over 25 years, there has so far been little theoretical insight regarding the many unusual low temperature properties of GGG. Here we investigate GGG in zero magnetic field using mean-field theory. We reproduce the spin liquid-like correlations and, most importantly, explain the positions of the sharp peaks seen in powder neutron diffraction experiments. We show that it is crucial to treat accurately the long-range nature of the magnetic dipolar interactions to allow for a determination of the small exchange energy scales involved in the selection of the experimental ordering wave vector. Our results show that the incommensurate order in GGG is classical in nature, intrinsic to the microscopic spin Hamiltonian and not caused by weak disorder.

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http://dx.doi.org/10.1103/PhysRevLett.97.267203DOI Listing

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