Normal mode splitting is observed in a cavity QED system in which nitrogen vacancy centers in diamond nanocrystals are coupled to whispering gallery modes in a silica microsphere. The composite nanocrystal-microsphere system takes advantage of the exceptional spin properties of nitrogen vacancy centers as well as the ultrahigh quality factor of silica microspheres. The observation of the normal mode splitting indicates that the dipole optical interaction between the relevant nitrogen vacancy center and whispering gallery mode has reached the strong coupling regime of cavity QED.
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http://dx.doi.org/10.1021/nl061342r | DOI Listing |
J Chem Theory Comput
December 2024
Max Planck Institute for the Structure and Dynamics of Matter, Luruper Ch 149, Hamburg 22761, Germany.
High-harmonic generation (HHG) is a nonlinear process in which a material sample is irradiated by intense laser pulses, causing the emission of high harmonics of incident light. HHG has historically been explained by theories employing a classical electromagnetic field, successfully capturing its spectral and temporal characteristics. However, recent research indicates that quantum-optical effects naturally exist or can be artificially induced in HHG, such as entanglement between emitted harmonics.
View Article and Find Full Text PDFNanophotonics
June 2024
Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, E-28049 Madrid, Spain.
The full information about the interaction between a quantum emitter and an arbitrary electromagnetic environment is encoded in the so-called spectral density. We present an approach for describing such interaction in any coupling regime, providing a Lindblad-like master equation for the emitter dynamics when coupled to a general nanophotonic structure. Our framework is based on the splitting of the spectral density into two terms.
View Article and Find Full Text PDFEntropy (Basel)
October 2024
Department of Physics and Astronomy and Institute for Quantum Science and Engineering, Texas A&M University, College Station, TX 77843-4242, USA.
We propose boson sampling from a system of coupled photons and Bose-Einstein condensed atoms placed inside a multi-mode cavity as a simulation process testing the quantum advantage of quantum systems over classical computers. Consider a two-level atomic transition far-detuned from photon frequency. An atom-photon scattering and interatomic collisions provide interactions that create quasiparticles and excite atoms and photons into squeezed entangled states, orthogonal to the atomic condensate and classical field driving the two-level transition, respectively.
View Article and Find Full Text PDFEntropy (Basel)
October 2024
Faculdade de Física, Universidade Federal do Pará, Belém 66075-110, Brazil.
Charged quasiparticles, which are constrained to move on a plane, interact by means of electromagnetic (EM) fields which are not subject to this constraint, living, thus, in three-dimensional space. We have, consequently, a hybrid situation where the particles of a given system and the EM fields (through which they interact) live in different dimensions. Pseudo-Quantum Electrodynamics (PQED) is a U(1) gauge field theory that, despite being strictly formulated in two-dimensional space, precisely describes the real EM interaction of charged particles confined to a plane.
View Article and Find Full Text PDFChem Asian J
November 2024
Research Institute for Electronic Science (RIES), Hokkaido University, North 20 West 10, Kita ward, Sapporo, Hokkaido, 001-0020, Japan.
Chemistry has traditionally focused on the synthesis of desired compounds, with organic synthesis being a key method for obtaining target molecules. In contrast, self-assembly -where molecules spontaneously organize into well-defined structures- has emerged as a powerful tool for fabricating intricate structures. Self-assembly was initially studied in biological systems but has been developed for synthetic methods, leading to the field of supramolecular chemistry, where non-covalent interactions/bonds guide molecular assembly.
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