The interaction of ultrashort laser pulses with matter is a topic of growing interest. In particular, recent developments on free-electron lasers have opened an unexplored field in which many interesting physical phenomena are to be expected. Since hydrodynamic descriptions of the interaction process need a microscopic "input," a quantum statistical theory of energy absorption by matter is required. We present a kinetic theory of collisional absorption in dense plasmas and analyze the electron-ion collision frequency in warm dense aluminum in dependence on laser frequency and temperature.
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http://dx.doi.org/10.1103/PhysRevE.73.066406 | DOI Listing |
Nanoscale
January 2025
Department of Chemistry, Faculty of Science, Kyushu University, 744 Motooka, Nishi-ku, Fukuoka 819-0395, Japan.
We report photodissociation processes and spectral measurements upon photoabsorption of size-selected cationic silver clusters, Ag, stored in an ion trap. The experiment shows that small clusters ( ≲ 15) dissociate upon one-photon absorption, whereas larger ones require multiple photons up to five in the present study. The emergence of multi-photon processes is attributed to collisional cooling in the presence of a buffer helium gas in the trap, which competes with size-dependent dissociation rates.
View Article and Find Full Text PDFInteractions between magma oceans and overlying atmospheres on young rocky planets leads to an evolving feedback of outgassing, greenhouse forcing, and mantle melt fraction. Previous studies have predominantly focused on the solidification of oxidized Earth-similar planets, but the diversity in mean density and irradiation observed in the low-mass exoplanet census motivate exploration of strongly varying geochemical scenarios. We aim to explore how variable redox properties alter the duration of magma ocean solidification, the equilibrium thermodynamic state, melt fraction of the mantle, and atmospheric composition.
View Article and Find Full Text PDFRev Sci Instrum
August 2024
ISTP-CNR, Institute for Plasma Science and Technology, Corso Stati Uniti 4, 35127 Padova, Italy.
The Thermal Helium Beam (THB) is a diagnostic for simultaneously measuring the electron temperature and density profiles of the plasma edge and scrape off layer (SOL). It exploits the line ratio technique of selected He line intensities, emitted by He gas puffed inside the plasma, to locally estimate the plasma properties through a dedicated collisional radiative model (CRM). Standard THB diagnostics used in nuclear fusion devices measure three HeI emission lines: 667.
View Article and Find Full Text PDFPhys Rev E
May 2024
Lawrence Livermore National Laboratory, Livermore, California 94550, USA.
We provide analytic expressions for the effective Coulomb logarithm for inverse bremsstrahlung absorption which predict significant corrections to the Langdon effect and overall absorption rate compared to previous estimates. The calculation of the collisional absorption rate of laser energy in a plasma by the inverse bremsstrahlung mechanism usually makes the approximation of a constant Coulomb logarithm. We dispense with this approximation and instead take into account the velocity dependence of the Coulomb logarithm, leading to a more accurate expression for the absorption rate valid in both classical and quantum conditions.
View Article and Find Full Text PDFFaraday Discuss
August 2024
Department of Chemistry and Biochemistry, University of Maryland College Park, College Park, Maryland 20742, USA.
Collisions of optically centrifuged CO molecules with = 244-282 ( = 22 800-30 300 cm) are investigated with high-resolution transient IR absorption spectroscopy to reveal collisional and orientational phenomena of molecules with hyper-thermal rotational energies. The optical centrifuge is a non-resonant optical excitation technique that uses ultrafast, 800 nm chirped pulses to drive molecules to extreme rotational states through sequential Raman transitions. The extent of rotational excitation is controlled by tuning the optical bandwidth of the excitation pulses.
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