We use Shannon's definition of information to develop a theory to predict a photon-counting-based single-molecule experiment's ability to measure the desired property. We treat three phenomena that are commonly measured on single molecules: spectral fluctuations of a solvatochromic dye; assignment of the azimuthal dipole angle; determination of a distance by fluorescence resonant energy transfer using Förster's theory. We consider the effect of background and other "imperfections" on the measurement through the decrease in information.
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| http://www.ncbi.nlm.nih.gov/pmc/articles/PMC1995558 | PMC |
| http://dx.doi.org/10.1021/jp062192b | DOI Listing |
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