Vanadyl complexes of C or N-capped tripodal ligands, possessing distorted tetrahedral geometry at vanadium, serve as extremely active, thermally robust pro-catalysts for ethylene homo- and ethylene/propylene copolymerisation, whereas pseudo-octahedral pro-catalysts produce far lower activities.
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Vanadyl C and N-capped tris(phenolate) complexes: influence of pro-catalyst geometry on catalytic activity.
Chem Commun (Camb)
August 2006
Wolfson Materials and Catalysis Centre, School of Chemical Sciences and Pharmacy, University of East Anglia, Norwich, Norfolk NR4 7TJ, UK.
Vanadyl complexes of C or N-capped tripodal ligands, possessing distorted tetrahedral geometry at vanadium, serve as extremely active, thermally robust pro-catalysts for ethylene homo- and ethylene/propylene copolymerisation, whereas pseudo-octahedral pro-catalysts produce far lower activities.
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