Nonlinear terahertz response of -type GaAs.

Phys Rev Lett

Max-Born-Institut für Nichtlineare Optik und Kurzzeitspektroskopie, 12489 Berlin, Germany.

Published: May 2006

Excitation of an n-type GaAs layer by intense ultrashort terahertz pulses causes coherent emission at 2 THz. Phase-resolved nonlinear propagation experiments show a picosecond decay of the emitted field, despite the ultrafast carrier-carrier scattering at a sample temperature of 300 K. While the linear THz response is in agreement with the Drude response of free electrons, the nonlinear response is dominated by the super-radiant decay of optically inverted impurity transitions. A quantum mechanical discrete state model using the potential of the disordered impurities accounts for all experimental observations.

Download full-text PDF

Source
http://dx.doi.org/10.1103/PhysRevLett.96.187402DOI Listing

Publication Analysis

Top Keywords

nonlinear terahertz
4
response
4
terahertz response
4
response -type
4
-type gaas
4
gaas excitation
4
excitation n-type
4
n-type gaas
4
gaas layer
4
layer intense
4

Similar Publications

Low-temperature phase (β-form) barium borate (BBO) is one of the most important nonlinear crystals that has been widely used for optical second-harmonic generation (SHG), especially with femtosecond sources. There was growing interest in its applications in the direct generation of terahertz (THz) radiations, but it was hindered by the lack of knowledge of its basic properties in the THz range. In a recent study based on first-principles quantum chemistry calculation, we found that the theoretically calculated refractive indices of β-BBO in the THz frequency range do not agree with the previously reported values.

View Article and Find Full Text PDF

Terahertz (THz) parametric detection is a highly sensitive method that upconverts a THz wave into a near-infrared beam for detection. Lithium niobate has primarily been used as the nonlinear optical crystal in this approach. However, the frequency band with high parametric gain is limited, leading to increasing interest in other nonlinear optical crystals.

View Article and Find Full Text PDF

Graphene has unique properties paving the way for groundbreaking future applications. Its large optical nonlinearity and ease of integration in devices notably makes it an ideal candidate to become a key component for all-optical switching and frequency conversion applications. In the terahertz (THz) region, various approaches have been independently demonstrated to optimize the nonlinear effects in graphene, addressing a critical limitation arising from the atomically thin interaction length.

View Article and Find Full Text PDF

Terahertz Saturable Absorption across Charge Separation in Photoexcited Monolayer Graphene/MoS Heterostructure.

J Phys Chem Lett

January 2025

Key Laboratory of Materials Physics, Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences, Hefei 230031, China.

Unveiling the nonlinear interactions between terahertz (THz) electromagnetic waves and free carriers in two-dimensional materials is crucial for the development of high-field and high-frequency electronic devices. Herein, we investigate THz nonlinear transport dynamics in a monolayer graphene/MoS heterostructure using time-resolved THz spectroscopy with intense THz pulses as the probe. Following ultrafast photoexcitation, the interfacial charge transfer establishes a nonequilibrium carrier redistribution, leaving free holes in the graphene and trapping electrons in the MoS.

View Article and Find Full Text PDF

Collective modes in terahertz field response of disordered superconductors.

J Phys Condens Matter

January 2025

Department of Physics, Kent State University, Kent, OH 44242, United States of America.

We consider a problem of nonlinear response to an external electromagnetic radiation in conventional disordered superconductors which contain a small amount of weak magnetic impurities. We focus on the diffusive limit and use Usadel equation to analyze the excitation energy and dispersion relation of the collective modes. We determine the resonant frequency and dispersion of both amplitude (Schmidt-Higgs) and phase (Carlson-Goldman) modes for moderate strength of magnetic scattering.

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!