Influence of transient phonon relaxation on the Brillouin loss spectrum of nanosecond pulses.

Opt Lett

Department of Physics, University of Ottawa, 150 Louis Pasteur Street, Ottawa, Ontario K1N 6N5, Canada.

Published: April 2006

For pump-probe stimulated Brillouin scattering with a probe pulse of a few nanoseconds duration and with a finite DC level, the acoustic wave relaxation time varies with the pump power and the DC level. For a pump power of 1-6 mW, the acoustic wave relaxation changes from approximately 9 to 90 ns for polarization-maintaining fiber at a temperature of -40 degrees C for a 2 ns pulse width. When the pulse DC ratio of the probe varies from 10 to 20 dB, the acoustic relaxation time changes from 24 to 45 ns for single-mode fiber at 25 degrees C. This induces a power-increment spectral feature in the detected AC pump signal in the Brillouin loss spectrum of two temperature or strain sections, where both spectral components appeared at positions far from those related to the natural phonon relaxation time (approximately 10 ns) equivalent length. The theoretical calculations confirm the prolonged phonon relaxation.

Download full-text PDF

Source
http://dx.doi.org/10.1364/ol.31.000888DOI Listing

Publication Analysis

Top Keywords

phonon relaxation
12
relaxation time
12
brillouin loss
8
loss spectrum
8
acoustic wave
8
wave relaxation
8
pump power
8
relaxation
6
influence transient
4
transient phonon
4

Similar Publications

Ultrafast Charge Carrier Dynamics in Vanadium Dioxide, VO: Nonequilibrium Contributions to the Photoinduced Phase Transitions.

J Phys Chem Lett

January 2025

Department of Mechanical and Aerospace Engineering, University of Virginia, Charlottesville, Virginia 22904, United States.

Vanadium oxide (VO) is an exotic phase-change material with diverse applications ranging from thermochromic smart windows to thermal sensors, neuromorphic computing, and tunable metasurfaces. Nonetheless, the mechanism responsible for its metal-insulator phase transition remains a subject of vigorous debate. Here, we investigate the ultrafast dynamics of the photoinduced phase transition in VO under low perturbation conditions.

View Article and Find Full Text PDF

A new compound [Y(sq)(HO)] (Y-sq; sq = squarate (CO)) was prepared and structurally characterized. Since the RE-sq family (RE = Y, Dy, Yb, Lu) gave isostructural crystals, the objective of this study is to explore the effects of diamagnetic dilution on the SIM behavior through systematic investigation and comparison of diamagnetically diluted and undiluted forms. The 1%-Diluted Dy compounds, Dy@Y-sq and Dy@Lu-sq, showed AC magnetic susceptibility peaks without any DC bias field (), whereas undiluted Dy-sq showed no AC out-of-phase response under the same conditions.

View Article and Find Full Text PDF

The quantum-well-like two-dimensional lead-halide perovskites exhibit strongly confined excitons due to the quantum confinement and reduced dielectric screening effect, which feature intriguing excitonic effects. The ionic nature of the perovskite crystal and the "softness" of the lattice induce the complex lattice dynamics. There are still open questions about how the soft lattices decorate the nature of excitons in these hybrid materials.

View Article and Find Full Text PDF

Hot carrier dynamics in the BAPbBr/MoS heterostructure.

Nanoscale

January 2025

Department of Condensed Matter and Materials Physics, S. N. Bose National Centre for Basic Sciences, Block JD, Sector III, Salt Lake, Kolkata-700106, India.

Herein, we investigated the carrier-phonon relaxation process in a two-dimensional (2D) BAPbBr perovskite and its heterostructure with MoS. Energy transfer was observed in the van der Waals heterostructure of 2D perovskite and monolayer MoS, leading to enhancement in the photoluminescence intensity of MoS. Femtosecond pump-probe spectroscopy was used to study the carrier and lattice dynamics of pristine 2D materials and their heterostructure.

View Article and Find Full Text PDF

Since the initial publication on the first TiCT MXene in 2011, there has been a significant increase in the number of reports on applications of MXenes in various domains. MXenes have emerged as highly promising materials for various biomedical applications, including photothermal therapy (PTT), drug delivery, diagnostic imaging, and biosensing, owing to their fascinating conductivity, mechanical strength, biocompatibility and hydrophilicity. Through surface modification, MXenes can mitigate cytotoxicity, enhance biological stability, and improve histocompatibility, thereby enabling their potential use in biomedical applications.

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!