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Orientation-Dependent Anisotropic Desalination by Assembled Zeolite Nanotube Membranes.
Langmuir
January 2025
College of Physical Science and Technology, Yangzhou University, Yangzhou 225002, China.
Porous nanomaterials have shown great promise in many desalination applications. Zeolite nanotubes, featuring abundant but inhomogeneous nanopores on their surface, have been recently synthesized in experiments; however, their capacity for desalination is not yet understood. In this work, we use molecular dynamics simulations to investigate the capability of assembled zeolite nanotube membranes to perform in desalination applications due to their inherent multiscale porous properties.
View Article and Find Full Text PDFInfluence of Deposition Temperature on Cu-BDC Surface-Anchored Metal-Organic Framework Formation.
J Phys Chem C Nanomater Interfaces
January 2025
Furman University, Greenville, South Carolina 29613, United States.
Surface-anchored metal-organic frameworks (surMOFs) are crystalline, nanoporous, supramolecular materials mounted to substrates that have the potential for integration within device architectures relevant for a variety of electronic, photonic, sensing, and gas storage applications. This research investigates the thin film formation of the Cu-BDC (copper benzene-1,4-dicarboxylate) MOF system on a carboxylic acid-terminated self-assembled monolayer by alternating deposition of solution-phase inorganic and organic precursors. X-ray diffraction (XRD) and atomic force microscopy (AFM) characterization demonstrate that crystalline Cu-BDC thin films are formed via Volmer-Weber growth.
View Article and Find Full Text PDFInterfacial Constructing Poly(ionic liquids) on Nanoporous Block Copolymers for Antifouling Ultrafiltration.
Langmuir
January 2025
State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, Nanjing, Jiangsu 211816, People's Republic of China.
The remarkable flexibility in structural tunability and designability of poly(ionic liquids) (PILs) has garnered significant attention. Integration of PILs with membranes, novel properties, and functionalities is anticipated for applications in the fields of membrane separation. Here, we develop a facile method to prepare PIL-functionalized membranes in a one-step process by combining selective swelling-induced pore generation and ionic liquid functionalization.
View Article and Find Full Text PDFPatterning the Pore Orientation of Nanoporous Metal via Self-Organization in Flow Cells.
Adv Sci (Weinh)
January 2025
Department of Mechanical and Aerospace Engineering, The Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong.
Nanoporous metals, a class of free-standing, high specific-area materials, evolve from interface-controlled self-organization in a selective dissolution (e.g., dealloying).
View Article and Find Full Text PDFConfining Liquid Electrolytes in a Nitrogen-Rich Nanoporous Carbon Sponge for Superior Lithium-Ion Conduction.
ACS Appl Mater Interfaces
January 2025
State Key Laboratory of Materials-Oriented Chemical Engineering and College of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, P. R. China.
Solid-state Li-ion batteries are recognized as highly promising energy storage devices due to their ability to overcome issues related to the inferior cycle life and potential risks of traditional liquid Li-ion batteries. However, developing solid-state electrolytes with fast Li-ion conductivity continues to be a major challenge. In this study, we present a family of quasi-solid-state electrolytes (QSSEs) synthesized by confining liquid electrolytes within a N-rich porous carbon sponge, exhibiting superior Li-ion conduction for solid-state battery applications.
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