Electric field tuning of plasmonic response of nanodot array in liquid crystal matrix.

Nano Lett

Division of Engineering and Department of Physics, Brown University, 182 Hope Street, Box D, Providence, RI 02912, USA.

Published: October 2005

In this work we demonstrate the feasibility of electric-field tuning of the plasmonic spectrum of a novel gold nanodot array in a liquid crystal matrix. As opposed to previously reported microscopically observed near-field spectral tuning of individual gold nanoparticles, this system exhibits macroscopic far-field spectral tuning. The nanodot-liquid crystal matrix also displays strong anisotropic absorption characteristics, which can be effectively described as a collective ensemble within a composite matrix in the lateral dimension and a group of noninteracting individual particles in the normal direction. The effective medium model and the Mie theory are employed to describe the experimental results.

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http://dx.doi.org/10.1021/nl0513535DOI Listing

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