Experimental evidence of above-threshold photoemission in solids.

Phys Rev Lett

Istituto Nazionale per la Fisica della Materia and Dipartimento di Matematica e Fisica, Università Cattolica, I-25121 Brescia, Italy.

Published: January 2005

Nonlinear photoemission from a silver single crystal is investigated by femtosecond laser pulses in a perturbative regime. A clear observation of above-threshold photoemission in solids is reported for the first time. The ratio between the three-photon above-threshold and the two-photon Fermi edges is found to be 10(-4). This value constitutes the only available benchmark for theories aimed at understanding the mechanism responsible for above-threshold photoemission in solids.

Download full-text PDF

Source
http://dx.doi.org/10.1103/PhysRevLett.94.037601DOI Listing

Publication Analysis

Top Keywords

above-threshold photoemission
12
photoemission solids
12
experimental evidence
4
above-threshold
4
evidence above-threshold
4
photoemission
4
solids nonlinear
4
nonlinear photoemission
4
photoemission silver
4
silver single
4

Similar Publications

Femtosecond Polarization Shaping of Free-Electron Laser Pulses.

Phys Rev Lett

July 2023

Elettra-Sincrotrone Trieste, 34149 Basovizza, Trieste, Italy.

We demonstrate the generation of extreme-ultraviolet (XUV) free-electron laser (FEL) pulses with time-dependent polarization. To achieve polarization modulation on a femtosecond timescale, we combine two mutually delayed counterrotating circularly polarized subpulses from two cross-polarized undulators. The polarization profile of the pulses is probed by angle-resolved photoemission and above-threshold ionization of helium; the results agree with solutions of the time-dependent Schrödinger equation.

View Article and Find Full Text PDF

Spectroscopic photoemission microscopy is used to detect and quantify a ponderomotive shift in the energy of electrons that are emitted from a surface plasmon polariton focus. The focus is formed on an atomically flat Au(111) surface by an Archimedean spiral and is spatiotemporally separated from the circularly polarized light pulse used to excite the spiral. A spectroscopic analysis of electrons emitted from the focus exhibits a peaked above-threshold electron emission spectrum.

View Article and Find Full Text PDF

Spatial-resolved photoelectron spectra have been observed from plasmonic metallic nanostructure and flat metal surface by a combination of time-of-flight photoemission electron microscope and femtosecond laser oscillator. The photoemission's main contribution is at localized 'hot spots,' where the plasmonic effect dominates and multiphoton photoemission is confirmed as the responsible mechanism for emission in both samples. Photoelectron spectra from hot spots exponentially decay in high energy regimes, smearing out the Fermi edge in Au flat surface.

View Article and Find Full Text PDF

Attosecond Time Delay of Retrapped Resonant Ionization.

Phys Rev Lett

September 2018

Department of Physics, College of Science, Shantou University, Shantou, Guangdong 515063, China.

A recent ultrafast pump-probe technique has allowed measurement of time delays during photoemission in a variety of systems ranging from atoms and molecules to solids with unprecedented temporal resolution. However, identifying the underlying physics is still a challenge especially in complicated multichannel above-threshold ionization (ATI) experiments. Here we demonstrate that the time delays of different ionization pathways in ATI can be clearly resolved and extracted with a semiclassical statistical method.

View Article and Find Full Text PDF

We use subcycle time-resolved photoemission microscopy to unambiguously distinguish optically triggered electron emission (photoemission) from effects caused purely by the plasmonic field (termed "plasmoemission"). We find from time-resolved imaging that nonlinear plasmoemission is dominated by the transverse plasmon field component by utilizing a transient standing wave from two counter-propagating plasmon pulses of opposite transverse spin. From plasmonic foci on flat metal surfaces, we observe highly nonlinear plasmoemission up to the fifth power of intensity and quantized energy transfer, which reflects the quantum-mechanical nature of surface plasmons.

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!