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Strategic Nitrogen Site Alignment in Covalent Organic Frameworks for Enhanced Performance in Aqueous Zinc-Iodide Batteries.
Angew Chem Int Ed Engl
January 2025
Northeast Normal University, Department of Chemistry, Renmin Street 5268, 130024, Changchun, CHINA.
Aqueous zinc-iodine batteries (AZIBs) are gaining attention as next-generation energy storage systems due to their high theoretical capacity, enhanced safety, and cost-effectiveness. However, their practical application is hindered by challenges such as slow reaction kinetics and the persistent polyiodide shuttle effect. To address these limitations, we developed a novel class of covalent organic frameworks (COFs) featuring electron-rich nitrogen sites with varied density and distribution (N1-N4) along the pore walls.
View Article and Find Full Text PDFBalancing pH and Pressure Allows Boosting Voltage and Power Density for a H-I Redox Flow Battery.
ACS Appl Energy Mater
January 2025
Department of Chemical Engineering, Delft University of Technology, Van der Maasweg 9, 2629HZ Delft, The Netherlands.
The decoupled power and energy output of a redox flow battery (RFB) offers a key advantage in long-duration energy storage, crucial for a successful energy transition. Iodide/iodine and hydrogen/water, owing to their fast reaction kinetics, benign nature, and high solubility, provide promising battery chemistry. However, H-I RFBs suffer from low open circuit potentials, iodine crossover, and their multiphase nature.
View Article and Find Full Text PDFPhase-Engineered Bi-RuO Single-Atom Alloy Oxide Boosting Oxygen Evolution Electrocatalysis in Proton Exchange Membrane Water Electrolyzer.
Adv Mater
January 2025
Shenzhen Key Laboratory of Energy Electrocatalytic Materials, Guangdong Provincial Key Laboratory of New Energy Materials Service Safety, College of Materials Science and Engineering, Shenzhen University, Shenzhen, Guangdong, 518055, P. R. China.
Engineering nanomaterials at single-atomic sites can enable unprecedented catalytic properties for broad applications, yet it remains challenging to do so on RuO-based electrocatalysts for proton exchange membrane water electrolyzer (PEMWE). Herein, the rational design and construction of Bi-RuO single-atom alloy oxide (SAAO) are presented to boost acidic oxygen evolution reaction (OER), via phase engineering a novel hexagonal close packed (hcp) RuBi single-atom alloy. This Bi-RuO SAAO electrocatalyst exhibits a low overpotential of 192 mV and superb stability over 650 h at 10 mA cm, enabling a practical PEMWE that needs only 1.
View Article and Find Full Text PDFLocal Structure Regulation for Oxygen Redox and Structure Stability of P2-Type Cathodes.
Small
January 2025
Materials Genome Institute, Shanghai University, Shanghai, 200444, China.
The local structure plays a crucial role in oxygen redox reactions, which boosts the capacity of layered oxide cathodes for sodium-ion batteries. While studies on local structural ordering have primarily focused on the intra-layer ordering, there has been limited research on the inter-layer stacking for the layered cathode materials for sodium-ion batteries. In this work, the impact of the intra-layer and inter-layer local structural regulation on anionic kinetics and the structure stability are explored through experimental analysis and theoretical calculations.
View Article and Find Full Text PDFPasteurized waste milk vs. milk replacer at the same crude protein:metabolizable energy ratio with different energy sources (fat vs. lactose) to pre-weaning Holstein calves: Effects on growth performance, feeding behavior, and health.
PLoS One
January 2025
Department of Animal Sciences, Washington State University, Pullman, Washington, United States of America.
The improved growth performance of calves at weaning results from an effective pre-weaning feeding strategy. The type and pasteurization process of liquid feed are among the most variable feeding practices affecting calves' growth and health. In previous studies that compared waste milk (WM) vs.
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