We consider several stochastic processes corresponding to the same physical solid-on-solid deposition problem. Simplified models presenting the same (conditional) mean and variance for each process are also introduced as well as generalizations in terms of the deposition of blobs and probabilistic deposition rules. We compare the evolution of the roughness as a function of time for a three-parameter family that includes as limit cases the Family model and the Edwards-Wilkinson equation, showing that in all cases the derived models with the same mean and variance are indistinguishable from the originating models in terms of the evolution of the roughness. Finally, we show that although all the models studied belong to the same universality class, some relevant features such as the final surface roughness are reproduced only for models within a restricted class determined by sharing the same (conditional) mean and variance.
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http://dx.doi.org/10.1103/PhysRevE.70.011605 | DOI Listing |
Phys Rev E
December 2023
Instituto de Física, Universidade Federal Fluminense, Avenida Litorânea s/n, 24210-340 Niterói, Rio de Janeiro, Brazil.
We perform kinetic Monte Carlo simulations of film growth in simple cubic lattices with solid-on-solid conditions, Ehrlich-Schwoebel (ES) barriers at step edges, and a kinetic barrier related to the hidden off-plane diffusion at multilayer steps. Broad ranges of the diffusion-to-deposition ratio R, detachment probability per lateral neighbor, ε, and monolayer step crossing probability P=exp[-E_{ES}/(k_{B}T)] are studied. Without the ES barrier, four possible scaling regimes are shown as the coverage θ increases: nearly layer-by-layer growth with damped roughness oscillations; kinetic roughening in the Villain-Lai-Das Sarma (VLDS) universality class when the roughness is W∼1 (in lattice units); unstable roughening with mound nucleation and growth, where slopes of logW×logθ plots reach values larger than 0.
View Article and Find Full Text PDFPhys Rev E
February 2021
Institut für Angewandte Physik, Universität Tübingen, 72076 Tübingen, Germany.
Thin-film growth is investigated in two types of lattice gas models where substrate and film particles are different, expressed by unequal interaction energy parameters. The first is of solid-on-solid type, whereas the second additionally incorporates desorption, diffusion in the gas phase above the film and readsorption at the film (appropriate for growth in colloidal systems). In both models, the difference between particle-substrate and particle-particle interactions plays a central role for the evolution of the film morphology at intermediate times.
View Article and Find Full Text PDFACS Appl Mater Interfaces
November 2019
MESA+ Institute for Nanotechnology , University of Twente, 7500 AE Enschede , Overijssel , Netherlands.
Ceramic-based nanocomposites are a rapidly evolving research area as they are currently being used in a wide range of applications. Epitaxial vertically aligned nanocomposites (VANs) offer promising advantages over conventional planar multilayers as key functionalities are tailored by the strong coupling at their vertical interfaces. However, limited knowledge exists of which material systems are compatible in composite films and which types of structures are optimal for a given functionality.
View Article and Find Full Text PDFPhysica D
January 2018
Department of Mathematics, and Institute for Physical Science and Technology, and Center for Scientific Computation and Mathematical Modeling, University of Maryland, College Park, MD 20742.
By linking atomistic and mesoscopic scales, we formally show how a local steric effect can hinder crystal growth and lead to a buildup of adsorbed atoms (adatoms) on a supersaturated, (1+1)-dimensional surface. Starting from a many-adatom master equation of a kinetic restricted solid-on-solid (KRSOS) model with we heuristically extract a coarse-grained, mesoscale description that defines the motion of a line defect (i.e.
View Article and Find Full Text PDFPhys Rev E
August 2017
Department of Mathematics, Institute for Physical Science and Technology, and Center for Scientific Computation and Mathematical Modeling, University of Maryland, College Park, Maryland 20742, USA.
We describe the effect of kinetic interactions of adsorbed atoms in a mesoscale model of epitaxial growth without elasticity. Our goal is to understand how atomic correlations due to kinetics leave their signature in mechanisms governing the motion of crystal line defects (steps) at the nanoscale. We focus on the key atomistic processes related to external material deposition, desorption, and asymmetric energy barriers on a stepped surface.
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