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A Zn-doped SbTe flexible thin film with decoupled Seebeck coefficient and electrical conductivity band engineering.
Chem Sci
January 2025
Shenzhen Key Laboratory of Advanced Thin Films and Applications, Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province, State Key Laboratory of Radio Frequency Heterogeneous Integration, College of Physics and Optoelectronic Engineering, Shenzhen University Shenzhen Guangdong 518060 China
SbTe-based flexible thin films can be utilized in the fabrication of self-powered wearable devices due to their huge potential in thermoelectric performance. Although doping can significantly enhance the power factor value, the process of identifying suitable dopants is typically accompanied by numerous repeating experiments. Herein, we introduce Zn doping into thermally diffused p-type SbTe flexible thin films with a candidate dopant validated using the first-principles calculations.
View Article and Find Full Text PDFHumic Acid with Vertical Adsorption Conformation Enhanced the Transport of Petroleum Hydrocarbon-Contaminated Colloids.
Environ Sci Technol
January 2025
College of Marine and Environmental Science, Tianjin University of Science and Technology, Tianjin 300457, China.
Humic acid (HA) enhances colloidal transport in porous media, yet the mechanisms by which the HA adsorption conformation affects colloid transport remain unclear. This study investigated the influence of HA on the transport of petroleum-hydrocarbon-contaminated soil colloids (TPHs-SC) in saturated sand columns. The presence of TPHs on the colloidal surface occupied adsorption sites, hindering HA from forming a horizontal adsorption conformation, as observed on uncontaminated soil colloids (SC).
View Article and Find Full Text PDFPressure-Induced Engineering of Surface Oxygen Vacancies on Metal Oxides for Heterogeneous Photocatalysis.
J Am Chem Soc
January 2025
State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou 350108, China.
Oxygen vacancies (OVs) spatially confined on the surface of metal oxide semiconductors are advantageous for photocatalysis, in particular, for O-involved redox reactions. However, the thermal annealing process used to generate surface OVs often results in undesired bulk OVs within the metal oxides. Herein, a high pressure-assisted thermal annealing strategy has been developed for selectively confining desirable amounts of OVs on the surface of metal oxides, such as tungsten oxide (WO).
View Article and Find Full Text PDFPulmonary Morbidity in Congenital Diaphragmatic Hernia Survivors Treated at a Non-ECMO Center From 1998 to 2015: A Cross-Sectional Study.
Pediatr Pulmonol
January 2025
Department of Clinical Research, Faculty of Health sciences, University of Southern Denmark, Odense, Denmark.
Introduction: A main feature of CDH is lung hypoplasia and the related presentation of pulmonary hypertension and cardiac dysfunction. Multiple factors influence pulmonary status after CDH: degree of hypoplasia, ventilator-induced injury, altered growth and development of pulmonary structures, reduced diaphragm function and chest wall abnormalities. The evolution of pulmonary sequela in this population is still unclear.
View Article and Find Full Text PDFSynaptic cleft geometry modulates NMDAR opening probability by tuning neurotransmitter residence time.
Biophys J
January 2025
Department of Pharmacology, School of Medicine, University of California San Diego, CA 92093, USA; Department of Mechanical and Aerospace Engineering, University of California San Diego, CA 92093, USA. Electronic address:
Synaptic morphology plays a critical role in modulating the dynamics of neurotransmitter diffusion and receptor activation in interneuron communication. Central physical aspects of synaptic geometry, such as the curvature of the synaptic cleft, the distance between the presynaptic and postsynaptic membranes, and the surface area-to-volume ratio of the cleft, crucially influence glutamate diffusion and N-Methyl-D-Aspartate receptor (NMDAR) opening probabilities. In this study, we developed a stochastic model for receptor activation using realistic synaptic geometries.
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