Using positional data from videomicroscopy and applying the equipartition theorem for harmonic Hamiltonians, we determine the wave-vector-dependent normal mode spring constants of a two-dimensional colloidal model crystal and compare the measured band structure to predictions of the harmonic lattice theory. We find good agreement for both the transversal and the longitudinal modes. For q-->0, the measured spring constants are consistent with the elastic moduli of the crystal.
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http://dx.doi.org/10.1103/PhysRevLett.92.215504 | DOI Listing |
Phys Chem Chem Phys
January 2025
School of Mechanical and Electrical Engineering, Lanzhou University of Technology, Lanzhou, 730050, China.
Previous researchers have conducted extensive investigations on the impact of various working conditions on fatigue damage. However, further research is still needed to understand the underlying mechanism of how the excitation frequency of cyclic loading affects the fatigue life. This article systematically discloses the phononic origin of atomic scale fatigue resonance, focusing on single-layer molybdenum disulfide (SL MoS) as a prototypical material.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
Department of Physics, School of Physical Science and Engineering, Beijing Jiaotong University, Beijing 100044, China.
Two-dimensional (2D) materials with spontaneous polarization can exhibit large second-order nonlinear optical (NLO) effects. Here, we present a series of stable distorted monolayers by using first-principles calculations and lattice vibration analysis. The structural distortion leads to a lower polar symmetry, giving rise to intrinsic ferroelectricity with a Curie point up to room temperature.
View Article and Find Full Text PDFACS Nano
January 2025
Sauvage Laboratory for Smart Materials, School of Materials Science and Engineering, Harbin Institute of Technology (Shenzhen), Shenzhen 518055, China.
With the potential to surpass the Shockley-Queisser (S-Q) limitation for solar energy conversion, the bulk photovoltaic (BPV) effect, which is induced by the broken inversion symmetry of the lattice, presents prospects for future light-harvesting technologies. However, the development of BPV is largely limited by the low solar spectrum conversion efficiency of existing noncentrosymmetric materials with wide band gaps. This study reports that the strain-induced reduction of inversion symmetry can enhance the second-order nonlinear susceptibility (χ) of SnPSe crystals by an order of magnitude, which contributes to an extremely high value of 1.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
Laser Thermal Laboratory, Department of Mechanical Engineering, University of California, Berkeley, California 94720, United States.
J Synchrotron Radiat
January 2025
Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201204, People's Republic of China.
The combination of reversible angular dispersion-induced microbunching (ADM) and the rapid damping storage ring provides a storage-ring-based light source with the capability to produce longitudinal coherent radiation with a high repetition rate. This paper presents a prototype design for a test facility based on the study by Jiang et al. [Sci.
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