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Chemical upcycling of poly(bisphenol A carbonate) via sequential diamino-/methanolysis: A phosgeneless one-pot route to dimethyl dicarbamate esters.
J Hazard Mater
November 2024
Università degli Studi "Aldo Moro" di Bari, Dipartimento di Chimica, Campus Universitario, Via E. Orabona, 4, 70126 Bari, Italy; Centro Interdipartimentale di Ricerca su Metodologie e Tecnologie Ambientali (METEA), via Celso Ulpiani 27, 70126 Bari, Italy. Electronic address:
Waste poly(bisphenol A carbonate) (PC) is a potential source of harmful bisphenol A (BPA). In this study a new approach aiming to chemically valorize hazardous PC wastes is described. A one-pot process has been developed that allows to recover BPA from PC used as "phosgene equivalent" for the synthesis of dimethyl dicarbamates MeOCNH-R-NHCOMe.
View Article and Find Full Text PDFCharacterization of the Structure of Rice and Wheat Straw Pretreated with . AH.
ACS Omega
November 2024
School of Chemical Engineering, Xuzhou College of Industrial Technology, Xuzhou 221140, Jiangsu, China.
. AH pretreatment (PT) enhances the conversion and selectivity of RS and WS in supercritical methanolysis. In this work, we investigated how .
View Article and Find Full Text PDFLocalized Electron Redistribution in Methanol Molecules over the Sea Urchin-like Tricobalt Tetroxide/Copper Oxide Nanostructures for Fast Hydrogen Release.
ACS Appl Mater Interfaces
November 2024
School of Chemistry and Materials Engineering, Huizhou University, Huizhou 516007, China.
Catalytic methanolysis of ammonia borane (NHBH) is a prospective technology in the field of hydrogen energy in which hydrogen production and hydrogen storage can be integrated together. The splitting of the O-H bond is identified as the rate-determining step (RDS) in this reaction. Thus, a deep understanding of the relationship between the electronic structure of the catalyst, especially the localized electron density of active sites, and the breaking behaviors of the O-H bond is of extreme importance for the rational design of robust catalysts for the reaction.
View Article and Find Full Text PDFMorphology engineering of hollow core@shell structured CoO@CuO-NiO for fast hydrogen release from ammonia borane methanolysis.
J Colloid Interface Sci
February 2025
School of Chemistry and Materials Engineering, Huizhou University, Huizhou 516007, China. Electronic address:
Catalytic methanolysis of ammonia borane is an integrated hydrogen production/storage technology with bright prospects, while its wide application is impeded by the high-cost of catalysts. In this work, hollow core@shell structured (HCSS) CoO@CuO-NiO with a size of 300-500 nm and a shell thickness of ca. 100 nm has been designed for ammonia borane (NHBH) methanolysis for rapid hydrogen release.
View Article and Find Full Text PDFE. coli-Assisted Eco-Friendly Production of Biogenic Silver Cobalt Oxide (AgCoO) Nanoparticles: Methanolysis-Based Hydrogen Production, Wastewater Remediation, and Pathogen Control.
Microsc Res Tech
November 2024
Biology Department, Faculty of Science, King Khalid University, Abha, Saudi Arabia.
Herein, bacterial-assisted synthesis of AgCoO is carried out. In the first step, E. coli was separated from soil samples via the "serial dilution method.
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