We present a new exciton-based formalism for calculating the coherent response of asymmetric semiconductor multiple quantum well structures to ultrashort optical pulses valid to infinite order in the optical field and including the self-generated intraband fields. We use these equations to calculate and explain the oscillations with time delay of peaks in the spectrally resolved degenerate four-wave mixing signals from biased semiconductor superlattices, obtaining good agreement with experiment.
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http://dx.doi.org/10.1103/PhysRevLett.91.267402 | DOI Listing |
J Chem Theory Comput
June 2022
Institute of Physics, Lodz University of Technology, ul. Wolczanska 217/221, 93-005, Lodz, Poland.
We address the problem of intermolecular interaction energy calculations in molecular complexes with localized excitons. Our focus is on the correct representation of the dispersion energy. We derive an extended Casimir-Polder formula for direct computation of this contribution through second order in the intermolecular interaction operator .
View Article and Find Full Text PDFJ Phys Condens Matter
March 2016
A.V.Rzhanov Institute of Semiconductor Physics, Siberian Branch of the Russian Academy of Sciences, Novosibirsk 630090, Russia. Novosibirsk State Technical University, Novosibirsk 630073, Russia.
Using the Feynman-Dyson diagram technique, we study nonlinear polariton-polariton scattering in a two-dimensional micropillar-based optical superlattice with hexagonal symmetry. We demonstrate that both the emerging polariton chirality and the loop Feynman diagrams up to infinite order should be strictly accounted for in the evaluation of the self-energy of the system. Further, we explicitly show that in such a design the time of polariton scattering towards the Dirac points can be drastically decreased which can be used, for instance, in engineering novel classes of polariton lasers with substantially reduced thresholds.
View Article and Find Full Text PDFJ Chem Theory Comput
August 2014
Cherry L. Emerson Center for Scientific Computation, Emory University, 1515 Dickey Dr., Atlanta, Georgia 30322, United States.
We describe an extension of the conventional Fourier grid discrete variable representation (DVR) to the bound state problem of a particle with a position-dependent mass. An infinite order DVR, derived for a variable mass kinetic energy operator, coupled with an efficient grid contraction scheme yields essentially exact eigenvalues for a chosen grid spacing. Implementation of the method is shown to be very practical due to the fact that in a DVR no integral evaluation is necessary and that the resultant kinetic energy matrix is sparse.
View Article and Find Full Text PDFPhys Rev Lett
December 2003
Department of Physics, Lakehead University, Thunder Bay, Ontario, Canada P7B 5E1.
We present a new exciton-based formalism for calculating the coherent response of asymmetric semiconductor multiple quantum well structures to ultrashort optical pulses valid to infinite order in the optical field and including the self-generated intraband fields. We use these equations to calculate and explain the oscillations with time delay of peaks in the spectrally resolved degenerate four-wave mixing signals from biased semiconductor superlattices, obtaining good agreement with experiment.
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